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000641735 1001_ $$aMaschwitz, Timo$$b0
000641735 245__ $$aHow crystallization additives govern halide perovskite grain growth
000641735 260__ $$a[London]$$bSpringer Nature$$c2025
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000641735 520__ $$aThe preparation of perovskite solar cells from the liquid phase is a cornerstone of their immense potential. However, a clear relationship between the precursor ink and the formation of the resulting perovskite is missing. Established theories, such as heterogeneous nucleation and lead complex colloid formation, often prove unreliable, which has led to an overreliance on heuristics. Most high-performing perovskites use additives to control crystallization. Their role during crystallization is, however, elusive. Here, we provide evidence that typical crystallization additives do not predominantly impact the nucleation phase but rather facilitate coarsening grain growth by increasing ion mobility across grain boundaries. Drawing from the insights of our broad, interdisciplinary study that combines ex and in situ characterization methods, devices, simulations, and density function theory calculation, we propose a concept that proves valid for various additives and perovskite formulations. Moreover, we establish a direct link between additive engineering and perovskite post-processing, offering a unified framework for advancing material design and process engineering.
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000641735 536__ $$0G:(EU-Grant)951774$$aFOXES - Fully Oxide-based Zero-Emission and Portable Energy Supply (951774)$$c951774$$fH2020-EIC-FETPROACT-2019$$x3
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000641735 7001_ $$0P:(DE-H253)PIP1088631$$aMerten, Lena$$b1
000641735 7001_ $$aÜnlü, Feray$$b2
000641735 7001_ $$00009-0005-1387-0616$$aMajewski, Martin$$b3
000641735 7001_ $$aHaddadi Barzoki, Fatemeh$$b4
000641735 7001_ $$aWu, Zijin$$b5
000641735 7001_ $$aÖz, Seren Dilara$$b6
000641735 7001_ $$aKreusel, Cedric$$b7
000641735 7001_ $$aTheisen, Manuel$$b8
000641735 7001_ $$00000-0002-9666-1422$$aWang, Pang$$b9
000641735 7001_ $$aSchiffer, Maximilian$$b10
000641735 7001_ $$aBoccarella, Gianluca$$b11
000641735 7001_ $$aMarioth, Gregor$$b12
000641735 7001_ $$aWeidner, Henrik$$b13
000641735 7001_ $$aSchultheis, Sarah$$b14
000641735 7001_ $$aSchieferstein, Tim$$b15
000641735 7001_ $$aGidaszewski, Dawid$$b16
000641735 7001_ $$aJulliev, Zavkiddin$$b17
000641735 7001_ $$0P:(DE-H253)PIP1088034$$aKneschaurek, Ekaterina$$b18
000641735 7001_ $$0P:(DE-H253)PIP1096639$$aMunteanu, Valentin$$b19
000641735 7001_ $$0P:(DE-H253)PIP1014884$$aZaluzhnyy, Ivan$$b20
000641735 7001_ $$0P:(DE-H253)PIP1007852$$aBertram, Florian$$b21
000641735 7001_ $$aJaffrès, Anaël$$b22
000641735 7001_ $$aHe, Junjie$$b23
000641735 7001_ $$aAshurov, Nigmat$$b24
000641735 7001_ $$00000-0002-4023-2178$$aStolterfoht, Martin$$b25
000641735 7001_ $$aWolff, Christian M.$$b26
000641735 7001_ $$0P:(DE-H253)PIP1085895$$aUnger, Eva$$b27
000641735 7001_ $$aOlthof, Selina$$b28
000641735 7001_ $$aBrocks, Geert$$b29
000641735 7001_ $$00000-0002-3658-8497$$aTao, Shuxia$$b30
000641735 7001_ $$00000-0002-5422-7003$$aGrüninger, Helen$$b31
000641735 7001_ $$aRonsin, Olivier J. J.$$b32
000641735 7001_ $$00000-0002-9200-6623$$aHarting, Jens$$b33
000641735 7001_ $$00009-0006-9148-0514$$aKotthaus, Andreas F.$$b34
000641735 7001_ $$aKirsch, Stefan F.$$b35
000641735 7001_ $$aMathur, Sanjay$$b36
000641735 7001_ $$0P:(DE-H253)PIP1081858$$aHinderhofer, Alexander$$b37
000641735 7001_ $$0P:(DE-H253)PIP1008437$$aSchreiber, Frank$$b38
000641735 7001_ $$00000-0003-1084-316X$$aRiedl, Thomas$$b39
000641735 7001_ $$0P:(DE-H253)PIP1108432$$aBrinkmann, Kai Oliver$$b40$$eCorresponding author
000641735 773__ $$0PERI:(DE-600)2553671-0$$a10.1038/s41467-025-65484-7$$gVol. 16, no. 1, p. 9894$$n1$$p9894$$tNature Communications$$v16$$x2041-1723$$y2025
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