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@ARTICLE{Guo:640324,
author = {Guo, Weijia and Pang, Zixuan and Cai, Xiaoping and Xie,
Chaoqun and Zhang, Baojing and Akhtar, Farid and Feng,
Peizhong},
title = {3{D} reconstruction and corrosion resistance of porous
{Z}r-{A}l intermetallic via thermally-regulated rapid
self-exothermic reaction},
journal = {Journal of alloys and compounds},
volume = {1039},
issn = {0925-8388},
address = {Lausanne},
publisher = {Elsevier},
reportid = {PUBDB-2025-04775},
pages = {183300},
year = {2025},
note = {Waiting for fulltext},
abstract = {For environmental management purposes, industrial alkaline
waste streams are essential to be filtered effectively.
Here, porous Zr-Al intermetallic compounds were prepared
using a rapid self-exothermic reaction with a preventative
holding treatment. The pre-heating treatment for
thermal-adjustment accelerates the solid-state diffusion
kinetics and reduces the heat released by the thermal
explosion reaction (TE). The porous Zr-Al compounds were
structurally reconstructed using the 3D X-ray microscopy
(3D-XRM) technique, through which the porosity, pore
connectivity, and permeability properties were
semi-quantitatively analyzed in conjunction with the
reconstructed model. In-situ high-temperature synchrotron
X-ray diffraction (HT-SXRD) was employed to reveal the phase
constitution evolution as a function of temperature,
underpinning the effectiveness of the pre-heating treatment
and revealing the formation of thermo-dynamically stable
intermetallic phases. The complete reaction between Zr and
Al is facilitated by the pre-heating treatment, producing a
homogeneous pore-skeleton structure and inhibiting
microcrack formation with superior connectivity and
permeability properties. Consequently, optimal sample
570/700 shows excellent filtering properties due to the
uniformly distributed and inter-connected pores. The
superior corrosion resistance further evidences the
expedited passivation film formation, combining with the
homogeneous pore structure and stable intermetallic
composition, which altogether improves substrate protection
and mitigates electrochemical degradation processes. The
structure-function integrated porous Zr-Al provides a
meaningful path and shows the potential for filtration
applications of industrial wastewater/gas.},
cin = {DOOR ; HAS-User},
ddc = {540},
cid = {I:(DE-H253)HAS-User-20120731},
pnm = {6G3 - PETRA III (DESY) (POF4-6G3) / FS-Proposal: I-20240759
(I-20240759) / FS-Proposal: I-20240761 (I-20240761) /
SWEDEN-DESY - SWEDEN-DESY Collaboration
$(2020_Join2-SWEDEN-DESY)$},
pid = {G:(DE-HGF)POF4-6G3 / G:(DE-H253)I-20240759 /
G:(DE-H253)I-20240761 / $G:(DE-HGF)2020_Join2-SWEDEN-DESY$},
experiment = {EXP:(DE-H253)P-P21.1-20150101},
typ = {PUB:(DE-HGF)16},
doi = {10.1016/j.jallcom.2025.183300},
url = {https://bib-pubdb1.desy.de/record/640324},
}