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@ARTICLE{Azzolin:640318,
author = {Azzolin, Agata and Giovannetti, Gaia and Cannelli, Oliviero
and Guangyu, Fan and Ahsan, Md Sabbir and Colaizzi, Lorenzo
and Maansson, Erik and Tettenborn, Noah and Oberti, Linda
and Facciala, Davide and Frassetto, Fabio and Ciriolo, Anna
Grabriella and Lodi, Dario W. and Ashraf, Alia and Manzoni,
Christian and Martínez Vázquez, Rebeca and Devetta,
Michele and Osellame, Roberto and poletto, luca and Stagira,
Salvatore and Vozzi, Caterina and Mullins, Terence and
Wanie, Vincent and Trabattoni, Andrea and Calegari,
Francesca},
title = {{E}ngineering {H}igh-{O}rder {H}armonic {G}eneration
through {G}as {C}onfinement at {S}ub-{M}illimeter {L}engths},
journal = {JPhys photonics},
volume = {8},
number = {1},
issn = {2515-7647},
address = {Bristol},
publisher = {IOP Publishing},
reportid = {PUBDB-2025-04769},
pages = {015057},
year = {2025},
abstract = {Attosecond light sources based on high-order harmonic
generation (HHG) constitute to date the only table-top
solution for producing coherent broadband radiation covering
the spectral range from the extreme ultraviolet to the soft
X-rays. The so-called emission cutoff can be extended
towards higher photon energies by increasing the driving
wavelength at the expense of conversion efficiency. An
alternative route is to overdrive the process by using
higher laser intensities, with the challenging requirement
of interacting with higher plasma densities over short
propagation distances. Here, we address this challenge by
using a differentially pumped glass chip designed for
optimal gas confinement over sub-mm lengths. By driving HHG
with multicycle pulses at either 800 nm or 1500 nm, we
demonstrate a cutoff extension by a factor of two compared
to conventional phase matching approaches and surpassing the
present record using multicycle fields. Our
three-dimensional propagation simulations, in excellent
agreement with the experiment, confirm that gas confinement
is crucial since efficient phase matching of cutoff
harmonics occurs only for short propagation lengths.
Additionally, we show that the high photon energy component
is not only temporally confined to the leading edge of the
driving pulse, but also spatially confined in the near-field
to an off-axis contribution due to reshaping of the driving
field along propagation inside the medium. Our findings
contribute to the fundamental understanding of HHG across
different regimes.},
cin = {FS-ATTO},
ddc = {530},
cid = {I:(DE-H253)FS-ATTO-20170403},
pnm = {631 - Matter – Dynamics, Mechanisms and Control
(POF4-631) / DFG project G:(GEPRIS)390715994 - EXC 2056:
CUI: Tiefe Einblicke in Materie (390715994) / METRICS -
Element-selective impulsive electronic and vibrational
spectroscopy of iron-sulfur clusters (101106352) / DFG
project G:(GEPRIS)545611997 - Vermessung von chiralen
Transienten von Attosekunden bis Femtosekunden durch
ultraschnelle Spektroskopie (545611997) / SoftMeter -
Multi-messenger soft-field spectroscopy of molecular
electronics at interfaces (101076500)},
pid = {G:(DE-HGF)POF4-631 / G:(GEPRIS)390715994 /
G:(EU-Grant)101106352 / G:(GEPRIS)545611997 /
G:(EU-Grant)101076500},
experiment = {EXP:(DE-MLZ)NOSPEC-20140101},
typ = {PUB:(DE-HGF)16},
doi = {10.1088/2515-7647/ae4080},
url = {https://bib-pubdb1.desy.de/record/640318},
}