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@ARTICLE{Min:639799,
author = {Min, Chul Hee and Müller, S. and Choi, W. J. and Dudy, L.
and Zabolotnyy, V. and Heber, M. and Denlinger, J. D. and
Kang, C.-J. and Kalläne, M. and Wind, N. and Scholz, M. and
Lee, T. L. and Schlueter, C. and Gloskovskii, A. and Rienks,
E. D. L. and Hinkov, V. and Bentmann, H. and Kwon, Y. S. and
Reinert, F. and Kim, H.-D. and Rossnagel, K.},
title = {{P}olaronic {Q}uasiparticles in the {V}alence-{T}ransition
{C}ompound {T}m{S}e$_{1−x}${T}e$_x$},
journal = {Physical review letters},
volume = {135},
number = {18},
issn = {0031-9007},
address = {College Park, Md.},
publisher = {APS},
reportid = {PUBDB-2025-04673},
pages = {186501},
year = {2025},
abstract = {Exotic quasiparticle states have been proposed in
mixed-valent compounds exhibiting valence transitions.
However, clear spectroscopic evidence identifying these
states has remained elusive. Using synchrotron-based hard
x-ray and extreme ultraviolet photoemission spectroscopy, we
have probed the Tm 3𝑑 and 4𝑓 emissions in
TmSe$_{1−x}$Te$_x$, where a Te concentration-dependent
semimetal–insulator transition occurs alongside the
valence transition. Our photoemission results, which are
characteristic of the bulk, track this combined transition
across the critical concentration ($𝑥_𝑐$ =0.29).
Notably, our results reveal a noninteger valence for the
insulating phase and a novel quasiparticle excitation in the
semimetallic phase: a Holstein polaron that extends beyond
the standard periodic Anderson model},
cin = {FS DOOR-User / FS-SXQM / FS-PET-S},
ddc = {530},
cid = {$I:(DE-H253)FS_DOOR-User-20241023$ /
I:(DE-H253)FS-SXQM-20190201 / I:(DE-H253)FS-PET-S-20190712},
pnm = {632 - Materials – Quantum, Complex and Functional
Materials (POF4-632) / 6G3 - PETRA III (DESY) (POF4-6G3) /
FS-Proposal: I-20200225 (I-20200225) / DFG project
G:(GEPRIS)390858490 - EXC 2147: Komplexität und Topologie
in Quantenmaterialien (CT.QMAT) (390858490) / SFB 1170 C06 -
Topologische Phasen in Schwere-Fermionen-Isolatoren und
-Halbmetallen, sowie die Be-deutung von Zeitumkehr- und
Inversionssymmetrie (C06) (276846545) / SFB 1170 A01 -
Einfluss von Symmetrie und Korrelationseffekten in der
elektronischen Struktur epitaktischer topologischer
Isolatoren (A01) (276799616) / CALIPSOplus - Convenient
Access to Light Sources Open to Innovation, Science and to
the World (730872) / 05K19FK4 - Verbundprojekt 05K2019 -
QM-MBE-SXPES: Experimentelle Apparatur zur
Molekularstrahlepitaxie komplexer Quantenmaterialien für
Photoelektronenspektroskopie im Weichröntgenbereich am
Strahlrohr P04 von PETRA III. Teilprojekt 1.
(BMBF-05K19FK4)},
pid = {G:(DE-HGF)POF4-632 / G:(DE-HGF)POF4-6G3 /
G:(DE-H253)I-20200225 / G:(GEPRIS)390858490 /
G:(GEPRIS)276846545 / G:(GEPRIS)276799616 /
G:(EU-Grant)730872 / G:(DE-Ds200)BMBF-05K19FK4},
experiment = {EXP:(DE-H253)P-P04-20150101 / EXP:(DE-H253)P-P22-20150101},
typ = {PUB:(DE-HGF)16},
doi = {10.1103/72dv-ynm2},
url = {https://bib-pubdb1.desy.de/record/639799},
}