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@ARTICLE{Cherevotan:639633,
author = {Cherevotan, Arjun and Singh, Ashutosh Kumar and Yadav,
Anish and Maligal-Ganesh, Raghu V. and Raj, Jithu and
Pulparambil, Anu and Goud, Devender and Vinod, Chathakudath
P. and Peter, Sebastian C.},
title = {{M}etal deficiency tuned charge transfer in intermetallic
{N}i$_{2−x}${S}n (x = 0.37–0.65) enhances selective
conversion of furfural to furfuryl alcohol towards the
theoretical limit},
journal = {Journal of materials chemistry / A},
volume = {13},
number = {8},
issn = {2050-7488},
address = {London [u.a.]},
publisher = {RSC},
reportid = {PUBDB-2025-04590},
pages = {6042 - 6048},
year = {2025},
note = {Waiting for fulltext},
abstract = {Heterogeneous catalysis facilitated by intermetallic
nanoparticles has recently been the subject of increased
scrutiny, given the enhanced selectivity and stability they
bestow on many chemical reactions compared to their
monometallic components. This paper explores a series of
Ni–Sn (Ni$_{2−x}$Sn, where x = 0.65, 0.5, 0.37)
intermetallic compounds supported on a high-surface-area
support, SBA-15, as catalysts for the selective
hydrogenation of furfural to furfuryl alcohol. Rietveld
refinements of the X-ray diffraction data show catalysts
with mixed intermetallic phases that assist in the
catalysis. At the same time, X-ray photoelectron
spectroscopy (XPS) studies and X-ray absorption studies
indicate the role played by charge transfer from Sn to Ni
for the catalysis. Selectivity to the desired furfuryl
alcohol in all the intermetallic samples was high (>97\%),
but Ni1.35Sn had a relatively lower conversion than the
other intermetallic compounds.},
cin = {DOOR ; HAS-User},
ddc = {530},
cid = {I:(DE-H253)HAS-User-20120731},
pnm = {6G3 - PETRA III (DESY) (POF4-6G3) / INDIA-DESY - INDIA-DESY
Collaboration $(2020_Join2-INDIA-DESY)$},
pid = {G:(DE-HGF)POF4-6G3 / $G:(DE-HGF)2020_Join2-INDIA-DESY$},
experiment = {EXP:(DE-H253)P-P64-20150101},
typ = {PUB:(DE-HGF)16},
doi = {10.1039/D4TA06383J},
url = {https://bib-pubdb1.desy.de/record/639633},
}