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@ARTICLE{Das:639592,
author = {Das, Ashok and Layek, Rashbihari and Mukherjee, Shounak and
Tayal, Akhil and Banerjee, Aritra and Kumbhakar, Pathik and
Bandyopadhyay, Sudipta},
title = {{C}omparative {I}nvestigation of the {C}ritical {R}ole of
{M}n, {Z}n, and {M}n/{Z}n {C}o‐{D}oping in {M}odulating
{L}ocal {C}oordination {E}nvironment, {M}agnetic {B}ehavior,
and {S}upercapacitor {P}erformance of
$α$‐{C}u$_2${V}$_2${O}$_7$},
journal = {Physica status solidi / A},
volume = {222},
number = {22},
issn = {1862-6300},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {PUBDB-2025-04568},
pages = {2500491},
year = {2025},
note = {Waiting for fulltext},
abstract = {Mn-, Zn-, and Mn/Zn-doped α-Cu2V2O7 (CVO) samples are
synthesized to investigate the interplay between local
structural distortion, magnetic behavior, and
electrochemical performance. Structural analysis via X-ray
diffraction, X-ray absorption near edge structure, and
extended X-ray absorption fine structure, along with
vibrational studies using Raman spectroscopy, confirms the
substitutional incorporation of Mn and Zn at Cu sites.
Doping introduces increased asymmetry in CuO bond lengths
and bond angles, disrupting super-exchange pathways.
Temperature-dependent magnetization measurements reveal a
marginal decrease in the Néel temperature (TN) with Zn and
Mn/Zn co-doping, while field-dependent studies indicate
enhanced magnetic hysteresis and a notable zero-field-cooled
exchange bias. Electrochemical characterization highlights
the strong influence of local structure: the Mn/Zn-doped CVO
exhibits the highest Debye–Waller factors (σ2) for both
first and second coordination shells, reduced Cu
coordination number, and pronounced CuO1 and CuO2 bond
length variations. These distortions promote enhanced charge
storage, resulting in superior specific capacitance compared
to singly doped analogs. This study underscores the critical
role of the local coordination environment in simultaneously
tailoring the magnetic and electrochemical properties of
CVO-based electrode materials.},
cin = {DOOR ; HAS-User / FS-PET-S},
ddc = {530},
cid = {I:(DE-H253)HAS-User-20120731 /
I:(DE-H253)FS-PET-S-20190712},
pnm = {632 - Materials – Quantum, Complex and Functional
Materials (POF4-632) / 6G3 - PETRA III (DESY) (POF4-6G3) /
INDIA-DESY - INDIA-DESY Collaboration
$(2020_Join2-INDIA-DESY)$},
pid = {G:(DE-HGF)POF4-632 / G:(DE-HGF)POF4-6G3 /
$G:(DE-HGF)2020_Join2-INDIA-DESY$},
experiment = {EXP:(DE-H253)P-P64-20150101},
typ = {PUB:(DE-HGF)16},
doi = {10.1002/pssa.202500491},
url = {https://bib-pubdb1.desy.de/record/639592},
}