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@ARTICLE{Hinsley:639480,
author = {Hinsley, Gerard N. and Ngoi, Kuan Hoon and Sturm, Sebastian
and Rysov, Rustam and Kirner, Felizitas and Lapkin, Dmitry
and Singh, Shweta and Assalauova, Dameli and Sprung, Michael
and Wiek, Thomas and Gemming, Thomas and Lubk, Axel and
Müller-Caspary, Knut and Sturm, Elena V. and Vartanyants,
Ivan A.},
title = {{M}apping the three-dimensional structure of faceted gold
mesocrystals using coherent {X}-ray diffraction imaging},
journal = {Missing Journal / Fehlende Zeitschrift},
volume = {2},
reportid = {PUBDB-2025-04565},
pages = {100269 -},
year = {2026},
note = {Missing Journal: Newton (Newton) = 2950-6360 (import from
CrossRef, Journals: bib-pubdb1.desy.de)},
abstract = {Elucidating the structure-property relationship of
mesocrystals requires understanding the mutual arrangement
of the nanoparticles within their assembly. This, therefore,
requires characterization techniques capable of
non-destructively distinguishing the shape, position, and
orientation of the individual constituent nanoparticles in
three dimensions. This detailed structural analysis is
achieved here by using coherent X-ray diffraction imaging
(CXDI) complemented with angular X-ray cross-correlation
analysis (AXCCA) and electron microscopy. Three mesocrystals
are examined, each assembled from different-sized gold
octahedral nano-particles and functionalized with
ω-thiol-terminated polystyrene (PS-SH) of different
molecular weights. AXCCA provides information regarding the
ensemble-averaged mesocrystal lattice structure, such as the
symmetry, unit cell parameters, and the presence of
orientational disorder. CXDI complementarily enables the
precise identification of the shape and positions of
individual nanoparticles as well as revealing any structural
defects. Our results show that each mesocrystal has a nearly
perfect lattice structure with minimal defects and exhibits
an increased strain toward the surface.},
cin = {FS-PETRA-S / DOOR ; HAS-User / FS-PS},
cid = {I:(DE-H253)FS-PETRA-S-20210408 /
I:(DE-H253)HAS-User-20120731 / I:(DE-H253)FS-PS-20131107},
pnm = {631 - Matter – Dynamics, Mechanisms and Control
(POF4-631) / 6G3 - PETRA III (DESY) (POF4-6G3)},
pid = {G:(DE-HGF)POF4-631 / G:(DE-HGF)POF4-6G3},
experiment = {EXP:(DE-H253)P-P10-20150101},
typ = {PUB:(DE-HGF)16},
doi = {10.1016/j.newton.2025.100269},
url = {https://bib-pubdb1.desy.de/record/639480},
}