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000639383 1001_ $$0P:(DE-H253)PIP1019042$$aFrost, Mungo$$b0$$eCorresponding author
000639383 245__ $$aSynthesis of Gold Hydride at High Pressure and High Temperature
000639383 260__ $$aWeinheim$$bWiley-VCH$$c2025
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000639383 520__ $$aGold is an unreactive metal and its chemical interactions with hydrogen have only recently been explored. Here, we report the formation of gold hydride above 40 GPa and 2200 K in X-ray free electron laser heated diamond anvil cells using various hydrocarbons as hydrogen sources. Above 40 GPa, a hexagonal phase emerges close to the gold melting point, corresponding to a hydride with stoichiometry mathematical equation, with mathematical equation increasing from 0 to near 1 with pressure from 40 to 80 GPa. This is a high-temperature phase which reverts to face centered cubic gold on cooling to 295 K. Accompanying DFT-MD simulations are in excellent agreement with experiment and reveal the structure to consist of an hexagonal close packed gold lattice with atomic hydrogen disordered in the interstices. The hydrogen is superionic and exhibits high diffusivity through the crystalline gold lattice. Our results present the first solid-state binary compound of gold and hydrogen.
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000639383 7001_ $$aAbraham, Kilian$$b1
000639383 7001_ $$0P:(DE-H253)PIP1015299$$aGoncharov, Alexander F.$$b2
000639383 7001_ $$0P:(DE-H253)PIP1021535$$aMcWilliams, R. Stewart$$b3
000639383 7001_ $$0P:(DE-H253)PIP1016653$$aHusband, Rachel J.$$b4
000639383 7001_ $$0P:(DE-H253)PIP1107613$$aAndrzejewski, Michal$$b5
000639383 7001_ $$0P:(DE-H253)PIP1001646$$aAppel, Karen$$b6
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000639383 7001_ $$0P:(DE-H253)PIP1102001$$aCeleste, Anna$$b11
000639383 7001_ $$0P:(DE-H253)PIP1087596$$aEdmund, Eric$$b12
000639383 7001_ $$aHartley, Nicholas J.$$b13
000639383 7001_ $$0P:(DE-H253)PIP1019654$$aGlazyrin, Konstantin$$b14
000639383 7001_ $$0P:(DE-H253)PIP1005340$$aGraafsma, Heinz$$b15
000639383 7001_ $$aJaisle, Nicolas$$b16
000639383 7001_ $$0P:(DE-H253)PIP1013606$$aKonôpková, Zuzana$$b17
000639383 7001_ $$0P:(DE-H253)PIP1006959$$aLaurus, Torsten$$b18
000639383 7001_ $$0P:(DE-H253)PIP1081528$$aLin, Yu$$b19
000639383 7001_ $$0P:(DE-H253)PIP1026549$$aMassani, Bernhard$$b20
000639383 7001_ $$0P:(DE-H253)PIP1080963$$aSchörner, Maximilian$$b21
000639383 7001_ $$aSchulze, Maximilian$$b22
000639383 7001_ $$0P:(DE-H253)PIP1017102$$aStrohm, Cornelius$$b23
000639383 7001_ $$0P:(DE-H253)PIP1087110$$aTang, Minxue$$b24
000639383 7001_ $$0P:(DE-H253)PIP1102560$$aYounes, Zena$$b25
000639383 7001_ $$aSteinle-Neumann, Gerd$$b26
000639383 7001_ $$0P:(DE-H253)PIP1010888$$aRedmer, Ronald$$b27
000639383 7001_ $$0P:(DE-H253)PIP1009803$$aGlenzer, Siegfried H.$$b28
000639383 773__ $$0PERI:(DE-600)2011836-3$$a10.1002/anie.202505811$$gVol. 64, no. 38, p. e202505811$$n38$$pe202505811$$tAngewandte Chemie / International edition$$v64$$x1433-7851$$y2025
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