Home > Publications database > Constraints on magnetism and correlations in RuO$_2$ from lattice dynamics and Mössbauer spectroscopy > print

001     638200
005     20251015213848.0
024 7 _ |a 10.1016/j.xcrp.2025.102852
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100 1 _ |a Yumnam, George
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245 _ _ |a Constraints on magnetism and correlations in RuO$_2$ from lattice dynamics and Mössbauer spectroscopy
260 _ _ |a Maryland Heights, MO
|c 2025
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520 _ _ |a We provide experimental evidence for the absence of a magnetic moment in bulk RuO$_2$, a candidate altermagnetic material, by using a combination of Mössbauer spectroscopy, nuclear forward scattering, inelastic X-ray and neutron scattering, and density functional theory calculations. Using complementary Mössbauer and nuclear forward scattering, we determine the Ru magnetic hyperfine splitting to be negligible. Inelastic X-ray and neutron scattering-derived lattice dynamics of RuO$_2$ are compared to density functional theory calculations of varying flavors. Comparisons among theory with experiments indicate that electronic correlations, rather than magnetic order, are key in describing the lattice dynamics.
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700 1 _ |a Raghuvanshi, Parul R.
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700 1 _ |a Budai, John D.
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700 1 _ |a Bocklage, Lars
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700 1 _ |a Abernathy, Douglas
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700 1 _ |a Cheng, Yongqiang
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700 1 _ |a Said, Ayman
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700 1 _ |a Mazin, Igor I.
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700 1 _ |a Zhou, Haidong
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700 1 _ |a Frandsen, Benjamin A.
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700 1 _ |a Parker, David S.
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700 1 _ |a Lindsay, Lucas R.
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700 1 _ |a Cooper, Valentino R.
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700 1 _ |a Manley, Michael E.
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700 1 _ |a Hermann, Raphael
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773 _ _ |a 10.1016/j.xcrp.2025.102852
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