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@ARTICLE{Mikhailova:637655,
author = {Mikhailova, Daria and Avdoshenko, Stanislav M. and Avdeev,
Maxim and Hanfland, Michael and Schwarz, Ulrich and Prots,
Yurii and Sarapulova, Angelina and Glazyrin, Konstantin and
Dubrovinsky, Leonid and Senyshyn, Anatoliy and Engel, Jens
and Ehrenberg, Helmut and Tsirlin, Alexander A.},
title = {{M}etallization without {C}harge {T}ransfer in
{C}u{R}e{O}$_4$ {P}errhenate under {P}ressure},
journal = {Inorganic chemistry},
volume = {64},
number = {12},
issn = {0020-1669},
address = {Washington, DC},
publisher = {American Chemical Society},
reportid = {PUBDB-2025-03881},
pages = {6010 - 6022},
year = {2025},
abstract = {Using high-pressure synchrotron X-ray diffraction combined
with Raman spectroscopy and density-functional calculations,
we determined the sequence of the pressure-induced
transformations in CuReO$_4$. At 1.5 GPa, the lattice
symmetry changes from I4$_1$cd to I4$_1$/a with the
transformation of isolated ReO$_4$-tetrahedra into infinite
chains of ReO$_6$-octahedra. The second, isosymmetric
transition at 7 GPa leads to the formation of a NbO$_2$-type
structure with the octahedral oxygen coordination for both
Cu$^{1+}$ and Re$^{7+}$ cations. Both transitions are of the
first order and accompanied by discontinuities in the
unit-cell volume of 7 and 14\%, respectively.
Density-functional calculations predict the metallic state
of the high-pressure NbO$_2$-type phase of CuReO$_4$, and
this prediction is in-line with the disappearance of the
Raman signal above 7 GPa and visual observations
(darkness/reflection of the sample). This metallization is
caused by the increased bandwidth of both Cu 3d and Re 5d
bands without any significant charge transfer between Cu and
Re. At ambient pressure, the crystal structure of CuReO$_4$
is retained between 4 and 700 K (melting point), showing a
negative thermal expansion along the c-axis and a positive
expansion along the a-axis within the entire temperature
range.},
cin = {DOOR ; HAS-User / FS DOOR-User / FS-PETRA-D / XFEL-User},
ddc = {540},
cid = {I:(DE-H253)HAS-User-20120731 /
$I:(DE-H253)FS_DOOR-User-20241023$ /
I:(DE-H253)FS-PETRA-D-20210408 /
I:(DE-H253)XFEL-User-20170713},
pnm = {631 - Matter – Dynamics, Mechanisms and Control
(POF4-631)},
pid = {G:(DE-HGF)POF4-631},
experiment = {EXP:(DE-H253)D-B2-20150101},
typ = {PUB:(DE-HGF)16},
doi = {10.1021/acs.inorgchem.4c05051},
url = {https://bib-pubdb1.desy.de/record/637655},
}