TY - JOUR
AU - Mikhailova, Daria
AU - Avdoshenko, Stanislav M.
AU - Avdeev, Maxim
AU - Hanfland, Michael
AU - Schwarz, Ulrich
AU - Prots, Yurii
AU - Sarapulova, Angelina
AU - Glazyrin, Konstantin
AU - Dubrovinsky, Leonid
AU - Senyshyn, Anatoliy
AU - Engel, Jens
AU - Ehrenberg, Helmut
AU - Tsirlin, Alexander A.
TI - Metallization without Charge Transfer in CuReO<sub>4</sub> Perrhenate under Pressure
JO - Inorganic chemistry
VL - 64
IS - 12
SN - 0020-1669
CY - Washington, DC
PB - American Chemical Society
M1 - PUBDB-2025-03881
SP - 6010 - 6022
PY - 2025
AB - Using high-pressure synchrotron X-ray diffraction combined with Raman spectroscopy and density-functional calculations, we determined the sequence of the pressure-induced transformations in CuReO<sub>4</sub>. At 1.5 GPa, the lattice symmetry changes from I4<sub>1</sub>cd to I4<sub>1</sub>/a with the transformation of isolated ReO<sub>4</sub>-tetrahedra into infinite chains of ReO<sub>6</sub>-octahedra. The second, isosymmetric transition at 7 GPa leads to the formation of a NbO<sub>2</sub>-type structure with the octahedral oxygen coordination for both Cu<sup>1+</sup> and Re<sup>7+</sup> cations. Both transitions are of the first order and accompanied by discontinuities in the unit-cell volume of 7 and 14
LB - PUB:(DE-HGF)16
DO - DOI:10.1021/acs.inorgchem.4c05051
UR - https://bib-pubdb1.desy.de/record/637655
ER -