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@ARTICLE{zsoy:637653,
author = {Özsoy, Andaç and Gaudez, Steve and Hearn, William A. and
Baganis, Antonios and Hegedüs, Zoltán and Chen, Yunhui and
Rack, Alexander and Logé, Roland E. and Van Petegem,
Steven},
title = {{P}hase-{S}eparation-{D}riven {C}racking in {A}dditive
{M}anufacturing of {N}i-{C}u {A}lloy {S}ystems},
journal = {Additive manufacturing},
volume = {110},
issn = {2214-7810},
address = {Amsterdam [u.a.]},
publisher = {Elsevier},
reportid = {PUBDB-2025-03879},
pages = {104950},
year = {2025},
abstract = {This study investigates the cracking mechanism in additive
manufacturing of Ni-Cu multi-material combinations using
operando X-ray diffraction and imaging experiments during
laser powder-bed fusion (L-PBF) of CuCrZr and IN625. It is
shown that liquid immiscibility between the two alloy
systems stems from the interaction between Cu and the
alloying elements in IN625, causing both Cu-rich and Ni-rich
liquids to form with different freezing ranges.
Consequently, solidification cracking takes place due to the
large solidification range where the Ni-rich solid and
Cu-rich liquid co-exist. Guided by thermodynamic
calculations, it was identified that the highest crack
susceptibility occurs between 20 and $40 wt\%$
CuCrZr-IN625, which was further validated by printing
mixtures of the two alloys in different ratios. Operando
X-ray imaging and scanning electron microscopy
characterization revealed that the cracking occurred during
the terminal stage of solidification. It was observed that
the columnar grains of the Ni-rich primary solid separate
into cracks, where Cu-rich liquid regions persist over a
wide temperature range as the solidification of these
regions begin significantly later. It was concluded that the
mechanism of cracking explained in this study could be
extended to other Cu-Ni alloy combinations containing
elements that induce immiscibility when mixed with Cu during
fusion-based processing methods.},
cin = {DOOR ; HAS-User / FS-PETRA-D},
cid = {I:(DE-H253)HAS-User-20120731 /
I:(DE-H253)FS-PETRA-D-20210408},
pnm = {632 - Materials – Quantum, Complex and Functional
Materials (POF4-632) / 6G3 - PETRA III (DESY) (POF4-6G3) /
PSI-FELLOW-III-3i - International, Interdisciplinary $\&$
Intersectoral Postdoctoral Fellowships at the Paul Scherrer
Institut (884104) / FS-Proposal: I-20230515 EC
(I-20230515-EC)},
pid = {G:(DE-HGF)POF4-632 / G:(DE-HGF)POF4-6G3 /
G:(EU-Grant)884104 / G:(DE-H253)I-20230515-EC},
experiment = {EXP:(DE-H253)P-P21.2-20150101},
typ = {PUB:(DE-HGF)16},
doi = {10.1016/j.addma.2025.104950},
url = {https://bib-pubdb1.desy.de/record/637653},
}