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000633849 1001_ $$0P:(DE-H253)PIP1025978$$aBloss, Dana$$b0$$eCorresponding author
000633849 245__ $$aSite- and Energy-Selective Low-Energy Electron Emission by X-rays in the Aqueous Phase
000633849 260__ $$aWashington, DC$$bACS Publications$$c2025
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000633849 520__ $$aLow-energy-electron emission from resonant Auger final states via intermolecular Coulombic decay (RA-ICD) has previously been described as a promising scenario for controlling radiation damage for medical purposes, but it has so far only been observed in prototypical atomic and molecular van der Waals dimers and clusters. Here, we report the experimental observation of RA-ICD in an aqueous solution. We show that for solvated Ca2+ ions, the emission can be very efficiently controlled by tuning the photon energy of exciting X-rays to inner-shell resonances of the ions. Our results provide the next step from demonstrating RA-ICD in relatively simple prototype systems to understanding the relevance and potential applications of ICD in real-life scenarios.
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000633849 536__ $$0G:(DE-Ds200)BMBF-05K22RK1$$a05K22RK1 - Verbundprojekt 05K2022 - TRANSALP: Zeit- & winkelaufgelöste Spektroskopie an Proben in der flüssigen Phase. Teilprojekt 2: Aufbau Liquid Jet und KI-basierte Datenanalyse. (BMBF-05K22RK1)$$cBMBF-05K22RK1$$f05K22RK1$$x3
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000633849 7001_ $$0P:(DE-H253)PIP1097998$$aDupuy, Remi$$b1
000633849 7001_ $$0P:(DE-H253)PIP1017364$$aTrinter, Florian$$b2
000633849 7001_ $$0P:(DE-H253)PIP1083693$$aUnger, Isaak$$b3
000633849 7001_ $$0P:(DE-H253)PIP1092293$$aWalsh, Noelle$$b4
000633849 7001_ $$0P:(DE-H253)PIP1025903$$aOehrwall, Gunnar$$b5
000633849 7001_ $$0P:(DE-H253)PIP1099637$$aGolchert, Niklas$$b6
000633849 7001_ $$0P:(DE-H253)PIP1103578$$aKlassen, Gabriel$$b7
000633849 7001_ $$0P:(DE-H253)PIP1105915$$aKrone, Adrian Peter$$b8
000633849 7001_ $$0P:(DE-H253)PIP1103234$$aTerao, Yusaku$$b9
000633849 7001_ $$0P:(DE-H253)PIP1032785$$aViehmann, Johannes$$b10
000633849 7001_ $$0P:(DE-HGF)0$$aWülfing, Lasse$$b11
000633849 7001_ $$0P:(DE-H253)PIP1098291$$aRichter, Clemens$$b12
000633849 7001_ $$0P:(DE-H253)PIP1095694$$aButtersack, Tillmann$$b13
000633849 7001_ $$0P:(DE-H253)PIP1027260$$aCederbaum, Lorenz$$b14
000633849 7001_ $$0P:(DE-H253)PIP1008114$$aHergenhahn, Uwe$$b15
000633849 7001_ $$0P:(DE-H253)PIP1083875$$aBjoerneholm, Olle$$b16
000633849 7001_ $$0P:(DE-H253)PIP1010716$$aEhresmann, Arno$$b17
000633849 7001_ $$0P:(DE-H253)PIP1017360$$aHans, Andreas$$b18$$eCorresponding author
000633849 773__ $$0PERI:(DE-600)1472210-0$$a10.1021/jacs.5c06436$$gVol. 147, no. 25, p. 22115 - 22120$$n25$$p22115 - 22120$$tJournal of the American Chemical Society$$v147$$x0002-7863$$y2025
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