TY - JOUR
AU - An, Siyu
AU - Karger, Leonhard
AU - Müller, Philipp
AU - Lin, Jing
AU - Vasala, Sami
AU - Baran, Volodymyr
AU - Dreyer, Sören L.
AU - Zhang, Ruizhuo
AU - Ulusoy, Fatih
AU - Kondrakov, Aleksandr
AU - Janek, Juergen
AU - Brezesinski, Torsten
TI - Exploring calcium pillaring of O3-type NaNi<sub>0.9</sub>Ti<sub>0.1</sub>O<sub>2</sub> cathodes to advance Na-ion battery technology
JO - The chemical engineering journal
VL - 509
SN - 1385-8947
CY - Amsterdam
PB - Elsevier
M1 - PUBDB-2025-02386
SP - 160939
PY - 2025
N1 - ISSN 1385-8947 not unique: **2 hits**.
AB - NaNi<sub>0.9</sub>Ti<sub>0.1</sub>O<sub>2</sub> (NNTO), a promising sodium-ion cathode material, is capable of delivering high specific capacities but is compromised by structural degradation at high potentials and poor redox stability. Herein, we introduced varying amounts of Ca<sup>2+</sup> as pillaring ions into the intercalation sites of NNTO to examine their effect on structure and electrochemical performance. Laboratory X-ray diffraction and charge/discharge testing identified Na<sub>0.95</sub>Ca<sub>0.025</sub>Ni<sub>0.9</sub>Ti<sub>0.1</sub>O<sub>2</sub> (CaNNTO) as the optimal composition in terms of interlayer spacing, rate capability, and cycling stability. Specifically, the capacity retention after 200 cycles improved from 27 to 48
LB - PUB:(DE-HGF)16
DO - DOI:10.1016/j.cej.2025.160939
UR - https://bib-pubdb1.desy.de/record/633260
ER -