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@ARTICLE{Sundermann:633257,
author = {Sundermann, Martin and Harder, Manuel and Said, Ayman H.
and Keimer, Bernhard and Gretarsson, Hlynur},
title = {{D}ispersion-compensated {R}owland spectrometer:
implications for uranium {VB}-{RIXS}},
journal = {Journal of synchrotron radiation},
volume = {33},
number = {1},
issn = {0909-0495},
address = {Chester},
publisher = {IUCr},
reportid = {PUBDB-2025-02383},
pages = {218 - 226},
year = {2026},
abstract = {The total energy resolution (ΔE$_{tot}$) of a valence-band
resonant inelastic X-ray scattering (VB-RIXS) instrument
serves as an important point of reference in an otherwise
complex field. Since VB-RIXS is a flux-limited technique, a
pragmatic approach to reducing ΔE$_{tot}$ is often
required—the specifications of a spectrometer should be
matched with a comparable incident bandwidth (ΔE$_i$) and
the source size contribution (focal point) should be
negligible. Although it advocates for a good efficiency,
this approach is in many places already limited by
count-rates. Here we follow a recent trend emerging in soft
X-ray VB-RIXS and look at the performance of our tender
X-ray Rowland spectrometer (Gretarsson et al., 2020) when
being exposed to a source with a large linear dispersion
(higher flux). Detailed ray tracing work, performed at the U
M5-edge (3551 eV), finds that the intrinsic resolution of
the Rowland spectrometer (ΔE$_a$) can be obtained if the
linear dispersion of the source matches the spectrometer's,
but opposite in sign—here ΔE$_i$ does not matter. This
finding is supported by experimental data where ΔE$_{tot}$
= 48 meV (ΔE$_a$ = 44 meV) was recently achieved.
Furthermore, we demonstrate that the dispersion rate can be
tuned, ensuring the method's applicability to other atomic
edges.},
cin = {FS-PETRA-S},
ddc = {550},
cid = {I:(DE-H253)FS-PETRA-S-20210408},
pnm = {632 - Materials – Quantum, Complex and Functional
Materials (POF4-632) / 6G3 - PETRA III (DESY) (POF4-6G3)},
pid = {G:(DE-HGF)POF4-632 / G:(DE-HGF)POF4-6G3},
experiment = {EXP:(DE-H253)P-P01-20150101},
typ = {PUB:(DE-HGF)16},
doi = {10.1107/S1600577525010318},
url = {https://bib-pubdb1.desy.de/record/633257},
}