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@ARTICLE{Rosenberger:632249,
author = {Rosenberger, Paul and Darmawan, Andri and Fedchenko, Olena
and Tkach, Olena and Chernov, Serhii V. and Kutnyakhov,
Dmytro and Hoesch, Moritz and Scholz, Markus and Rossnagel,
Kai and Pentcheva, Rossitza and Schoenhense, Gerd and
Elmers, Hans-Joachim and Mueller, Martina},
title = {{S}pin polarization of the two-dimensional electron gas at
the {E}u{O}/{S}r{T}i{O}$_3$ (001) interface},
journal = {Physical review materials},
volume = {9},
number = {6},
issn = {2475-9953},
address = {College Park, MD},
publisher = {APS},
reportid = {PUBDB-2025-02175},
pages = {064401},
year = {2025},
abstract = {Spin-polarized two-dimensional electron gases (2DEGs) are
of particular interest for functional oxide electronics
applications. The redox-created 2DEG residing on the
strontium titanate, SrTiO3 (STO), side of a europium
monoxide (EuO)/SrTiO3 (001) interface is expected to be
significantly spin polarized due to the proximity to the
strong (7ππ΅/π.π’.) Heisenberg ferromagnet EuO. We
apply magnetic circular dichroism in the angular
distribution (MCDAD) of photoemitted electrons to
investigate whether and how the induced spin polarization of
the 2DEG depends on the dimensionality of the overlaying EuO
layer. The experimental data are complemented by density
functional theory calculations with a Hubbard π term
(DFT+π). We show that the EuO/STO interfacial 2DEG is
spin polarized even for ultrathin EuO overlayers, starting
at an EuO threshold thickness of only two monolayers.
Additional EuO monolayers even increase the induced magnetic
Ti moment and thus the spin polarization of the 2DEG. Our
results and the potential to enhance the magnetic order of
EuO by other proximity effects indicate that the
EuO/STO(001) interface is an ideal template for creating
(multi-)functional spin-polarized 2DEGs for application in
oxide electronics.},
cin = {DOOR ; HAS-User / FS-PET-D / FS-FLASH-O / FS-FLASH /
FS-SXQM},
ddc = {530},
cid = {I:(DE-H253)HAS-User-20120731 / I:(DE-H253)FS-PET-D-20190712
/ I:(DE-H253)FS-FLASH-O-20160930 /
I:(DE-H253)FS-FLASH-20140814 / I:(DE-H253)FS-SXQM-20190201},
pnm = {631 - Matter β Dynamics, Mechanisms and Control
(POF4-631) / 6G3 - PETRA III (DESY) (POF4-6G3)},
pid = {G:(DE-HGF)POF4-631 / G:(DE-HGF)POF4-6G3},
experiment = {EXP:(DE-H253)P-P04-20150101},
typ = {PUB:(DE-HGF)16},
doi = {10.1103/PhysRevMaterials.9.064401},
url = {https://bib-pubdb1.desy.de/record/632249},
}