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@ARTICLE{Keshri:632247,
author = {Keshri, Aryan and Das, Prasanna and Devaraj, Nayana and
Chowdhury, Sourav and Dey, Jayjit Kumar and Ojha, Sunil and
Gupta, Pushpendra and Hoesch, Moritz and Afaneh, Feras and
Roul, Basanta and Venkatesan, Thirumalai and Saha, Bivas and
Narayan, Awadhesh and Bibes, Manuel and Das, Sujit},
title = {{U}nlocking {E}xceptional {N}egative {V}alency and {S}pin
{R}econstruction in {N}on‐{C}ollinear
{A}nti‐{F}erromagnetic {A}ntiperovskite {M}n$_3${N}i{N}
{F}ilm},
journal = {Advanced functional materials},
volume = {35},
number = {32},
issn = {1616-301X},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {PUBDB-2025-02173},
pages = {2500655},
year = {2025},
note = {Waiting for fulltext},
abstract = {Antiperovskite manganese nitrides have intriguing magnetic
and electronic properties that are not well understood. Just
as their perovskite oxide counterparts, they are expected to
display properties tunable through epitaxial strain
engineering, which has barely been explored yet. Here, three
notable contributions are made to the understanding and
tuning of these fascinating materials, focusing on
Mn$_3$NiN. First, combining X-ray spectroscopy measurements
and first-principles calculations, an unusually large
negative oxidation state of Ni$^{3−}$is reported. Second,
a substantial shift of the antiferromagnetic ordering
temperature by 116 K, from 266 to 150 K, is reported by
growing Mn3NiN films on different substrates. This shift is
due to the mixed contributions of ferrimagnetic and
antiferromagnetic phases. Third, a plasmonic signature with
a high optical extinction coefficient in the infrared to
visible range is exhibited, tunable by different substrates.
The findings suggest that Mn3NiN has significant potential
in antiferromagnetic spintronics, and plasmonics, expanding
the scope of new materials for electromagnetic
field-controlled plasmonics, piezo spintronics, and
multicaloric applications.},
cin = {FS DOOR-User / FS-PET-S},
ddc = {530},
cid = {$I:(DE-H253)FS_DOOR-User-20241023$ /
I:(DE-H253)FS-PET-S-20190712},
pnm = {631 - Matter – Dynamics, Mechanisms and Control
(POF4-631) / 6G3 - PETRA III (DESY) (POF4-6G3) / INDIA-DESY
- INDIA-DESY Collaboration $(2020_Join2-INDIA-DESY)$},
pid = {G:(DE-HGF)POF4-631 / G:(DE-HGF)POF4-6G3 /
$G:(DE-HGF)2020_Join2-INDIA-DESY$},
experiment = {EXP:(DE-H253)P-P04-20150101},
typ = {PUB:(DE-HGF)16},
doi = {10.1002/adfm.202500655},
url = {https://bib-pubdb1.desy.de/record/632247},
}