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@ARTICLE{Chowdhury:627901,
author = {Chowdhury, Subhadip and Mukhopadhyay, Mrinmay Kumar and
Sanyal, Milan and Bhunia, Satyaban and Satpati, Biswarup and
Giri, Rajendra P and Bharatiya, B. and Shen, Chen and
Murphy, Bridget M.},
title = {{I}nvestigation on the formation of two dimensional
perovskite nanostructures at the water surface through self
initiated reaction},
journal = {Scientific reports},
volume = {15},
issn = {2045-2322},
address = {[London]},
publisher = {Springer Nature},
reportid = {PUBDB-2025-01676},
pages = {6216},
year = {2025},
note = {BMBF/05K16FK1/05K19FK2/ 05K21FK3 research grants for
financing the LISA instrument},
abstract = {The emerging class of hybrid organic-inorganic perovskites
(HOIPs) has exhibited fascinating properties for a wide
range of technological applications. With halide ions, HOIPs
have provided novel optoelectronic devices including
efficient solar cells and with pseudohalide anions-like
formate (HCOO$^−$), enigmatic electromagnetic properties
have been obtained in HOIPs. Large-scale synthesis of such
2D HOIP films is of immense importance for the advancement
of its application as solar materials. We have shown using
in-situ X-ray measurements that the Langmuir monolayer of
perovskite can be formed at the air-water interface by
spreading stearic acid molecules on the water subphase
having (C$_4$H$_9$NH$_3$)$_2$PbBr$_4$ molecules. The 2D lead
formate perovskite films are formed at the air-water
interface through a self-initiated reaction and the in-situ
X-ray scattering and ex-situ Raman spectroscopy measurements
revealed this reaction process. The spreading of lipid
molecules having positive and negative head-group charges as
surfactants over the water surface shows that the formation
of perovskite nanofilms at the air-water interface
specifically requires the presence of HCOO$^−$ head-group
of stearic acid. In this room temperature interfacial
reaction, formate anions come from the stearic acid
monolayer present on the water surface and completely
replace bromines in the perovskite present in water subphase
to form (BA)$_2$Pb(HCOO)$_4$ at the air-water interface. Our
results show an easy route for large-scale synthesis of 2D
pseudohalide perovskites.},
cin = {FS DOOR-User / FS-PETRA-D},
ddc = {600},
cid = {$I:(DE-H253)FS_DOOR-User-20241023$ /
I:(DE-H253)FS-PETRA-D-20210408},
pnm = {632 - Materials – Quantum, Complex and Functional
Materials (POF4-632) / 6G3 - PETRA III (DESY) (POF4-6G3) /
INDIA-DESY - INDIA-DESY Collaboration
$(2020_Join2-INDIA-DESY)$},
pid = {G:(DE-HGF)POF4-632 / G:(DE-HGF)POF4-6G3 /
$G:(DE-HGF)2020_Join2-INDIA-DESY$},
experiment = {EXP:(DE-H253)P-P08-20150101},
typ = {PUB:(DE-HGF)16},
pubmed = {39979302},
UT = {WOS:001428038400045},
doi = {10.1038/s41598-024-78259-9},
url = {https://bib-pubdb1.desy.de/record/627901},
}