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@ARTICLE{Kotla:627883,
author = {Kotla, Surya Rohith and Ramakrishnan, Sitaram and Schaller,
Achim M. and Rekis, Toms and Eisele, Claudio and Bao, Jin-Ke
and Noohinejad, Leila and de Laitre, Geoffroy and de
Boissieu, Marc and van Smaalen, Sander},
title = {{D}eciphering the commensurately modulated monoclinic phase
of {R}b$_2${Z}n{C}l$_4$ at low temperatures},
journal = {Journal of solid state chemistry},
volume = {345},
issn = {0022-4596},
address = {Orlando, Fla.},
publisher = {Academic Press},
reportid = {PUBDB-2025-01658},
pages = {125226},
year = {2025},
abstract = {The ferroelectric phase III of Rb$_2$ZnCl$_4$ is stable
below $T_c$ = 192 K. It is known to be a threefold
superstructure of the centrosymmetric high-temperature
structure, with space group $P2_1 cn$. Below $T_L$ = 70 K,
phase IV exists as a sixfold superstructure. We report the
crystal structure of phase IV with monoclinic symmetry $Cc$
(b unique), while a structure model with symmetry $Pn$ (c
unique) leads to an almost equally good, yet significantly
worse fit to the diffraction data. Employing the superspace
approach to these commensurately modulated structures
results in modulation waves that follow the two-dimensional
irreducible representation $T_1$ of $P2_1 cn$, albeit with
different order parameter directions defining $Cc$ and $Pn$
symmetries, consistent with the literature. Standard tools
of crystal-chemical analysis indicate that the sixfold
superstructure is more stable than the threefold
superstructure of phase III. However, crystal-chemical
arguments cannot distinguish between the correct
superstructure model with space group $Cc$ ($b$ unique) and
the incorrect superstructure model with symmetry $Pn$ ($c$
unique) for phase IV. New crystal chemical tools are
required, in order to attain a meaningful understanding of
superstructure formation.},
cin = {FS DOOR-User / FS-PET-D},
ddc = {540},
cid = {$I:(DE-H253)FS_DOOR-User-20241023$ /
I:(DE-H253)FS-PET-D-20190712},
pnm = {631 - Matter – Dynamics, Mechanisms and Control
(POF4-631) / 6G3 - PETRA III (DESY) (POF4-6G3) /
FS-Proposal: I-20190544 (I-20190544) / DFG project
G:(GEPRIS)406658237 - Aperiodische Kristalle: Struktur,
Dynamik und elektronische Eigenschaften (406658237)},
pid = {G:(DE-HGF)POF4-631 / G:(DE-HGF)POF4-6G3 /
G:(DE-H253)I-20190544 / G:(GEPRIS)406658237},
experiment = {EXP:(DE-H253)P-P24-20150101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:001425621500001},
doi = {10.1016/j.jssc.2025.125226},
url = {https://bib-pubdb1.desy.de/record/627883},
}