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@ARTICLE{Levcenko:626497,
author = {Levcenko, Sergiu and Ritter, Konrad and Falk, Hans and
Pfeiffelmann, Timo and Trefflich, Lukas and Welter, Edmund
and Grundmann, Marius and Schnohr, Claudia},
title = {{R}ole of sample thickness and self-absorption effects in
simultaneous {XEOL}-{XAS} measurements on single crystalline
{Z}n{O} and {G}a{N}},
journal = {Physical review research},
volume = {7},
number = {2},
issn = {2643-1564},
address = {College Park, MD},
publisher = {APS},
reportid = {PUBDB-2025-01450},
pages = {023066},
year = {2025},
abstract = {The x-ray excited optical luminescence (XEOL) for defect
and near band edge (NBE) transitions combinedwith
simultaneous x-ray absorption measurements are
experimentally and theoretically studied on single
crystalline ZnO and GaN across the Zn and Ga K edges,
respectively, in a wide range of sample
thicknesses.Increasing the sample thickness leads to the
appearance of an inverted line shape and negative edge jump
forthe XEOL defect response, whereas the line shape of the
XEOL NBE edge remains positive. A one-dimensionaltransport
model is developed, which includes experimental geometry,
the creation of x-ray generated excitations,diffusion and
recombination of the carriers, and reabsorption of x-ray
fluorescence and XEOL photons. Themodel calculations
reproduce the experimentally observed changes of the edge
shape in the XEOL spectra causedby variation of the sample
thickness and reveal surface recombination and optical
absorption as the main factorsdetermining the XEOL edge
shape for a given sample thickness.},
cin = {FS DOOR-User / FS-PET-S},
ddc = {530},
cid = {$I:(DE-H253)FS_DOOR-User-20241023$ /
I:(DE-H253)FS-PET-S-20190712},
pnm = {632 - Materials – Quantum, Complex and Functional
Materials (POF4-632) / 6G3 - PETRA III (DESY) (POF4-6G3) /
FS-Proposal: II-20200005 (II-20200005) / FS-Proposal:
I-20220601 (I-20220601) / 05K19OL1 - Identifizierung von
Defekten durch elementspezifische Anregung optischer
Lumineszenz (BMBF-05K19OL1)},
pid = {G:(DE-HGF)POF4-632 / G:(DE-HGF)POF4-6G3 /
G:(DE-H253)II-20200005 / G:(DE-H253)I-20220601 /
G:(DE-Ds200)BMBF-05K19OL1},
experiment = {EXP:(DE-H253)P-P65-20150101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:001472569200002},
doi = {10.1103/PhysRevResearch.7.023066},
url = {https://bib-pubdb1.desy.de/record/626497},
}