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000626290 1001_ $$0P:(DE-H253)PIP1091862$$aInoue, Ichiro$$b0$$eCorresponding author
000626290 245__ $$aHigh-intensity X-ray pump-monochromatic X-ray probe technique across time zero
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000626290 520__ $$aA femtosecond pump–probe technique, capable of probing transient changes in intense X-ray-excited matter with monochromatic X-ray pulses and accessing data for both positive and negative delay times, is proposed. The application of this technique to single-crystal silicon revealed ultrafast X-ray-induced electron excitation occurring on a timescale of 10 fs, along with the delayed onset of atomic disordering relative to the electronic excitation. This technique will pave the way for atom-specific multidimensional spectroscopy and diagnostics of exotic states of matter created by X-ray irradiation with sophisticated probing techniques, such as single-crystal diffraction, inelastic scattering, X-ray Thomson scattering, and absorption spectroscopy. 
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000626290 7001_ $$0P:(DE-H253)PIP1023988$$aOsaka, Taito$$b1
000626290 7001_ $$0P:(DE-H253)PIP1020328$$aTkachenko, Victor$$b2
000626290 7001_ $$0P:(DE-HGF)0$$aHara, Toru$$b3
000626290 7001_ $$aKapcia, Konrad J.$$b4
000626290 7001_ $$0P:(DE-H253)PIP1009952$$aInubushi, Yuichi$$b5
000626290 7001_ $$0P:(DE-HGF)0$$aKawaguchi, Shogo$$b6
000626290 7001_ $$aYamada, Jumpei$$b7
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000626290 7001_ $$aYabashi, Makina$$b9
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