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@ARTICLE{Elmers:626184,
author = {Elmers, Hans-Joachim and Tkach, O. and Lytvynenko, Y. and
Yogi, P. and Schmitt, M. and Biswas, D. and Liu, J. and
Chernov, S. V. and Nguyen, Quynh and Hoesch, M. and
Kutnyakhov, D. and Wind, N. and Wenthaus, L. and Scholz, M.
and Rossnagel, K. and Gloskovskii, A. and Schlueter, C. and
Winkelmann, A. and Haghighirad, A.-A. and Lee, T.-L. and
Sing, M. and Claessen, R. and Le Tacon, M. and Demsar, J.
and Schoenhense, Gerd and Fedchenko, O.},
title = {{C}hirality in the {K}agome {M}etal {C}s{V}$_3${S}b$_5$},
journal = {Physical review letters},
volume = {134},
number = {9},
issn = {0031-9007},
address = {College Park, Md.},
publisher = {APS},
reportid = {PUBDB-2025-01327},
pages = {096401},
year = {2025},
note = {restricted document, copyright restrictionsThis work was
funded by theDeutsche Forschungsgemeinschaft (DFG,
GermanResearch Foundation), Grant No.
TRR288–422213477(Projects B03, B04, and B08), and Grant
No. Scho341/16-1, through the Collaborative Research Center
SFB 1170ToCoTronics (Project No. 258499086), through
theWürzburg-Dresden Cluster of Excellence on Complexityand
Topology in Quantum Matter ct.qmat (EXC 2147,Project No.
390858490), and by the BMBF (Projects05K22UM2, 05K22UM4, and
05K22WW1). Funding forthe instrument by the Federal Ministry
of Education andResearch (BMBF) under framework program ErUM
isgratefully acknowledged. We thank the Diamond LightSource
for providing beamtime at beamline I09. Weacknowledge DESY
(Hamburg, Germany) for the provisionof experimental
facilities. Parts of this research were carriedout at PETRA
III using beamlines P04 and P22. This workwas partially
funded by the Helmholtz Association IVF fundunder project
InterLabs-0002 “HELPFEL.},
abstract = {Using x-ray photoelectron diffraction (XPD) and
angle-resolved photoemission spectroscopy, we study
photoemission intensity changes related to changes in the
geometric and electronic structure in the kagome metal
CsV$_3$Sb$_5$ upon transition to an unconventional charge
density wave (CDW) state. The XPD patterns reveal the
presence of a chiral atomic structure in the CDW phase.
Furthermore, using circularly polarized x-rays, we have
found a pronounced nontrivial circular dichroism in the
angular distribution of the valence band photoemission in
the CDW phase, indicating a chirality of the electronic
structure. This observation is consistent with the proposed
orbital loop current order. In view of a negligible
spontaneous Kerr signal in recent magneto-optical studies,
the results suggest an antiferromagnetic coupling of the
orbital magnetic moments along the 𝑐 axis. While the
inherent structural chirality may also induce circular
dichroism, the observed asymmetry values seem to be too
large in the case of the weak structural distortions caused
by the CDW.},
cin = {DOOR ; HAS-User / FS-SXQM / FS-PETRA-S / FS-FLASH-O},
ddc = {530},
cid = {I:(DE-H253)HAS-User-20120731 / I:(DE-H253)FS-SXQM-20190201
/ I:(DE-H253)FS-PETRA-S-20210408 /
I:(DE-H253)FS-FLASH-O-20160930},
pnm = {632 - Materials – Quantum, Complex and Functional
Materials (POF4-632) / 6G3 - PETRA III (DESY) (POF4-6G3) /
DFG project G:(GEPRIS)422213477 - TRR 288: Elastisches
Tuning und elastische Reaktion elektronischer Quantenphasen
der Materie (ELASTO-Q-MAT) (422213477) / DFG project
G:(GEPRIS)444821420 - Elastische Kontrolle von
konkurrierenden Ordnungen in korrelierten Quantenmaterialien
(B03) (444821420) / DFG project G:(GEPRIS)444821616 -
Impuls-Mikroskopie von stark korrelierten Systemen unter
mechanischer Dehnung (B04) (444821616) / DFG project
G:(GEPRIS)444846624 - Ultraschnelle Spektroskopie und
Manipulation gekoppelter elektronischer/Gitter-Ordnungen
(B08) (444846624) / DFG project G:(GEPRIS)258499086 - SFB
1170: Topologische und korrelierte Elektronik in Ober- und
Grenzflächen ("ToCoTronics") (258499086) / DFG project
G:(GEPRIS)390858490 - EXC 2147: Komplexität und Topologie
in Quantenmaterialien (CT.QMAT) (390858490)},
pid = {G:(DE-HGF)POF4-632 / G:(DE-HGF)POF4-6G3 /
G:(GEPRIS)422213477 / G:(GEPRIS)444821420 /
G:(GEPRIS)444821616 / G:(GEPRIS)444846624 /
G:(GEPRIS)258499086 / G:(GEPRIS)390858490},
experiment = {EXP:(DE-H253)P-P04-20150101 / EXP:(DE-H253)P-P22-20150101 /
EXP:(DE-MLZ)External-20140101},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:40131065},
UT = {WOS:001458956900003},
doi = {10.1103/PhysRevLett.134.096401},
url = {https://bib-pubdb1.desy.de/record/626184},
}