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@ARTICLE{Vallinayagam:626083,
author = {Vallinayagam, Muthu and Nentwich, Melanie and Meyer, Dirk
C. and Zschornak, Matthias},
title = {{L}inearization routines for the parameter space concept to
determine crystal structures without {F}ourier inversion},
journal = {Journal of applied crystallography},
volume = {58},
number = {3},
issn = {0021-8898},
address = {Copenhagen},
publisher = {Munksgaard},
reportid = {PUBDB-2025-01288},
pages = {768 - 788},
year = {2025},
abstract = {We present the elaboration and first generally applicable
linearization routines of the parameter space concept (PSC)
for determining one-dimensionally projected structures of m
independent scatterers. This crystal determination approach
does not rely on Fourier inversion but rather considers all
structure parameter combinations consistent with available
diffraction data in a para- meter space of dimension m. The
method utilizes m structure-factor amplitudes or intensities
represented by piecewise analytic hyper-surfaces, to define
the acceptable parameter regions. By employing the
isosurfaces, the coordinates of the point scatterers are
obtained through the intersection of multiple isosur- faces.
This approach allows for the detection of all possible
solutions for the given structure-factor amplitudes in a
single derivation. Taking the resonant contrast into
account, the spatial resolution achieved by the presented
method may exceed that of traditional Fourier inversion, and
the algorithms can be significantly optimized by exploiting
the symmetry properties of the isosurfaces. The applied
one-dimensional projection demonstrates the efficiency of
the PSC linearization approach based on fewer reflections
than Fourier sums. The Monte Carlo simulations, using the
projections of various random two- and three-atom structure
examples, are presented to illustrate the universal
applicability of the proposed method. Furthermore, ongoing
efforts aim to enhance the efficiency of data handling and
to overcome current constraints, promising further
advancements in the capabilities and accuracy of the PSC
framework.},
cin = {IT},
ddc = {540},
cid = {I:(DE-H253)IT-20120731},
pnm = {611 - Fundamental Particles and Forces (POF4-611) / DFG
project G:(GEPRIS)442646446 - Parameter Space Concept als
Strukturlösungsmethodik für die Einkristalldiffraktometrie
(442646446)},
pid = {G:(DE-HGF)POF4-611 / G:(GEPRIS)442646446},
experiment = {EXP:(DE-MLZ)NOSPEC-20140101},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:40475935},
doi = {10.1107/S1600576725001955},
url = {https://bib-pubdb1.desy.de/record/626083},
}