Home > Publications database > Structure and properties of tubular structures based on the quaternary misfit layered compound Sm$_{1− x}$ Y$_x$S–TaS$_2$ > print

001     625723
005     20250715151536.0
024 7 _ |a 10.1039/D5RA00780A
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100 1 _ |a Hettler, Simon
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245 _ _ |a Structure and properties of tubular structures based on the quaternary misfit layered compound Sm$_{1− x}$ Y$_x$S–TaS$_2$
260 _ _ |a London
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520 _ _ |a Misfit layered compounds (MLCs) are incommensurate super-lattices made up of two repeating subunits and are promising for different applications due to the possibility of a synergetic combination of the properties of the employed sublayers. A means of fine-tuning a specific MLC is to alloy one of the elements in the system. In this study, quaternary MLCs made of Sm$_{1− x}$Y$_x$S–TaS$_2$ were successfully synthesized and the resulting structures were characterized in detail, with a specific focus on tubular structures. Owing to the small difference between the ionic radii of Sm and Y, the structure of the quaternary MLCs follows the one of pristine SmS–TaS$_2$, irrespective of the degree of alloying and with an anisotropic change of the lattice parameters up to a maximum of 2.7%. Nevertheless, microscopy, spectroscopy, and diffraction techniques allow us to reveal the impact of the composition on important characteristics of the MLC. Notably, for a specific composition, the ratio between the lattice parameters of the two subsystems adopts a value of 3 to 5, which could lead to a transition toward a commensurate superstructure.
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700 1 _ |a Furqan, Mohammad
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700 1 _ |a Sreedhara, M. B.
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700 1 _ |a Khadiev, Azat
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700 1 _ |a Tenne, Reshef
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700 1 _ |a Arenal, Raul
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773 _ _ |a 10.1039/D5RA00780A
|g Vol. 15, no. 13, p. 9605 - 9617
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