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000625583 1001_ $$aVinci, Doriana$$b0
000625583 245__ $$aCapturing ultrafast molecular motions and lattice dynamics in spin crossover film using femtosecond diffraction methods
000625583 260__ $$a[London]$$bSpringer Nature$$c2025
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000625583 520__ $$aA comprehensive insight into ultrafast dynamics of photo-switchable materials is desired for efficient control of material properties through light excitation. Here, we study a polycrystalline spin crossover thin film as a prototypical example and reveal the sequential photo-switching dynamics, from local molecular rearrangement to global lattice deformation. On the earliest femtosecond timescale, the local molecular structural rearrangement occurs within a constant unit-cell volume through a two-step process, involving initial Fe−ligand bond elongation followed by ligand rotation. The highly-oriented structure of the nanocrystalline films and the experimental geometry enables resolving the full anisotropic lattice structural dynamics in and out of the sample plane separately. While both molecular switching and lattice heating influence lattice volume, they exert varying degrees of impact at disparate time scales following photoexcitation. This study highlights the opportunities provided by Mega-electron-volt electron and X-ray free electron laser to advance the understanding of ultrafast dynamics of photo-switchable materials.
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000625583 7001_ $$aRidier, Karl$$b1
000625583 7001_ $$aQi, Fengfeng$$b2
000625583 7001_ $$aArdana-Lamas, Fernando$$b3
000625583 7001_ $$aZalden, Peter$$b4
000625583 7001_ $$aLiu, Lai Chung$$b5
000625583 7001_ $$aEklund, Tobias$$b6
000625583 7001_ $$aJakobsen, Mads Sielemann$$b7
000625583 7001_ $$aSchubert, Robin$$b8
000625583 7001_ $$aKhakhulin, Dmitry$$b9
000625583 7001_ $$aDeiter, Carsten$$b10
000625583 7001_ $$aBottin, Nicolas$$b11
000625583 7001_ $$aYousef, Hazem$$b12
000625583 7001_ $$avon Stetten, David$$b13
000625583 7001_ $$aŁaski, Piotr$$b14
000625583 7001_ $$00000-0002-8450-0955$$aKamiński, Radosław$$b15
000625583 7001_ $$aJarzembska, Katarzyna N.$$b16
000625583 7001_ $$aWallick, Rachel F.$$b17
000625583 7001_ $$aStensitzki, Till$$b18
000625583 7001_ $$avan der Veen, Renske M.$$b19
000625583 7001_ $$aMüller-Werkmeister, Henrike M.$$b20
000625583 7001_ $$aMolnár, Gábor$$b21
000625583 7001_ $$00000-0003-1590-7193$$aXiang, Dao$$b22
000625583 7001_ $$aMilne, Christopher$$b23
000625583 7001_ $$aLorenc, Maciej$$b24
000625583 7001_ $$0P:(DE-H253)PIP1018302$$aJiang, Yifeng$$b25$$eCorresponding author
000625583 773__ $$0PERI:(DE-600)2553671-0$$a10.1038/s41467-025-57202-0$$gVol. 16, no. 1, p. 2043$$n1$$p2043$$tNature Communications$$v16$$x2041-1723$$y2025
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