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000625325 1001_ $$0P:(DE-H253)PIP1100622$$aKumar, Rahul$$b0
000625325 245__ $$aCharacterization of the Spin-Frustration in Doubly Ordered Perovskite NaYbZnWO$_6$ Obtained by High-Pressure Synthesis
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000625325 520__ $$aWe present the high-pressure synthesis of a novel doubly ordered perovskite NaYbZnWO$_6$ composed of the rare earth magnetic Yb$^{3+}$ ions and its comprehensive magnetic characterization. The structure consists of alternating layers of Yb$^{3+}$ and Na$^+$ ions along the c-axis, with Yb$^{3+}$ ions forming slightly distorted two-dimensional (2D) square lattices of kite-shape (Yb$^{3+}$)4 units. Low-temperature magnetic susceptibility measurements indicate that the ground state of Yb$^{3+}$ can be described by an effective J$_{eff}$ = 1/2 Kramers doublet. Further, specific heat analysis reveals an internal magnetic field of the order of 1.48 K; however, magnetization data do not exhibit magnetic ordering down to 0.4 K. The spin exchanges of NaYbZnWO$_6$ evaluated by density functional theory (DFT) calculations unveil spin frustration in the compound. These findings suggest that NaYbZnWO$_6$ is a promising candidate for realizing a magnetically disordered quantum state.
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000625325 7001_ $$0P:(DE-H253)PIP1015084$$aBhat, Shrikant$$b1
000625325 7001_ $$00000-0001-9232-8289$$aKoo, Hyun-Joo$$b2
000625325 7001_ $$0P:(DE-HGF)0$$aNam, Kiwan$$b3
000625325 7001_ $$0P:(DE-HGF)0$$aKim, Seong-Hoon$$b4
000625325 7001_ $$0P:(DE-HGF)0$$aKim, Kee Hoon$$b5
000625325 7001_ $$00000-0002-2220-1124$$aWhangbo, Myung-Hwan$$b6
000625325 7001_ $$0P:(DE-H253)PIP1086024$$aAthinarayanan, Sundaresan$$b7$$eCorresponding author
000625325 773__ $$0PERI:(DE-600)1484438-2$$a10.1021/acs.inorgchem.4c04122$$gVol. 64, no. 8, p. 3677 - 3685$$n8$$p3677 - 3685$$tInorganic chemistry$$v64$$x0020-1669$$y2025
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