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| 001 | 625203 | ||
| 005 | 20250715151520.0 | ||
| 024 | 7 | _ | |a 10.1103/PhysRevB.111.104418 |2 doi |
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| 100 | 1 | _ | |a Hayashida, S. |0 0000-0003-0740-4852 |b 0 |e Corresponding author |
| 245 | _ | _ | |a Magnetic ground state of the dimer-based hexagonal perovskite Ba$_3$ZnRu$_2$O$_9$ |
| 260 | _ | _ | |a Woodbury, NY |c 2025 |b Inst. |
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| 520 | _ | _ | |a We investigate the magnetic ground state of single crystals of the ruthenium-dimer-based hexagonal perovskite Ba$_3$ZnRu$_2$O$_9$ using magnetic susceptibility and resonant inelastic x-ray scattering (RIXS) measurements. While a previous study on powder samples exhibited intriguing magnetic behavior, questions about whether the spin state within a Ru$_2$O$_9$ dimer is a conventional 𝑆=3/2 dimer or an orbital-selective 𝑆=1 dimer were raised. The RIXS spectra reveal magnetic excitations from Hund's intraionic multiplet and intradimer spin-triplet transitions. The observed transition energies of the Hund's intraionic multiplets align with the 𝑆=3/2 ground state, contrasting with the theoretically proposed orbital-selective 𝑆=1 dimer state. High-temperature magnetic susceptibility analysis confirms the realization of the spin 𝑆=3/2 dimer state, and the extracted intradimer coupling is consistent with the spin-triplet transition energy observed in the RIXS spectra. These results highlights the ability of “spectroscopic fingerprinting” by RIXS to determine the magnetic ground states of complex materials. |
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| 700 | 1 | _ | |a Matsumoto, Y. |0 0000-0001-8522-7113 |b 5 |
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