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100 1 _ |a Marotzke, Simon
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245 _ _ |a First experiments with ultrashort, circularly polarized soft x-ray pulses at FLASH2
260 _ _ |a Melville, NY
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500 _ _ |a Additional grant:Deutsche Forschungsgemeinschaft (DFG) - ProjectID 328545488 - TRR 227 “Ultrafast Spin Dynamics”.
520 _ _ |a Time-resolved absorption Spectroscopy as well as Magnetic Circular Dichroism with circularpolarized soft X-rays (XAS and XMCD) are powerful tools to probe electronic and magnetic dynamicsin magnetic materials in an element- and site selective manner. Employing these methods,groundbreaking results have been achieved for instance for magnetic alloys, which helped to fundamentallyadvance the field. The possibilities for ultrafast XAS and XMCD experiments, haverecently improved: In an upgrade of the free electron laser FLASH, a variable polarization afterburnerundulator at FLASH2 was installed in September 2023. This upgrade allows the generationof few tens of femtosecond short circularly polarized soft X-ray pulses covering the L2,3-edges of theimportant 3d transition metal elements. Here, we present first experimental results with circularlypolarized ultrashort X-ray pulses from the FL23 beamline employing XMCD at the L-edges of the3d elements, Co, Fe and Ni. We obtain significant XMCD, which hints to a degree of circular polarizationclose to 100%. Making use of the full pulse-length preserving monochromator capabilitiesof FL23 and an improved pump laser setup, FLASH offers important and efficient experimentalinfrastructure for ultrafast spin dynamics studies in 3d transition metals.
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700 1 _ |a Gupta, Deeksha
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700 1 _ |a Amrhein, Tim
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700 1 _ |a Vaskivskyi, Igor
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700 1 _ |a Knut, Ronny
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700 1 _ |a Engel, Dieter
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700 1 _ |a Braune, Markus
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700 1 _ |a Ilchen, Markus
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700 1 _ |a Savio, Sara
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700 1 _ |a Otto, Thorsten
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700 1 _ |a Tiedtke, Kai
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700 1 _ |a Scheppe, V.
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700 1 _ |a Rönsch-Schulenberg, Juliane
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700 1 _ |a Schneidmiller, Evgeny Alexanrdovich
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700 1 _ |a Schuessler-Langeheine, Christian
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700 1 _ |a Duerr, Hermann
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700 1 _ |a Beye, Martin
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700 1 _ |a Brenner, Guenter
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700 1 _ |a Pontius, Niko
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|e Corresponding author
770 _ _ |a Celebrating the work and the achievements of Jo Stöhr
773 _ _ |a 10.1063/4.0000298
|g Vol. 12, no. 3, p. 034301
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|t Structural dynamics
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