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@ARTICLE{Marotzke:622831,
author = {Marotzke, Simon and Gupta, Deeksha and Wang, Ru-Pan and
Pavelka, Martin and Dziarzhytski, Siarhei and von Korff
Schmising, Clemens and Jana, Somnath and Thielemann-Kuehn,
Nele and Amrhein, Tim and Weinelt, Martin and Vaskivskyi,
Igor and Knut, Ronny and Engel, Dieter and Braune, Markus
and Ilchen, Markus and Savio, Sara and Otto, Thorsten and
Tiedtke, Kai and Scheppe, V. and Rönsch-Schulenberg,
Juliane and Schneidmiller, Evgeny Alexanrdovich and
Schuessler-Langeheine, Christian and Duerr, Hermann and
Beye, Martin and Brenner, Guenter and Pontius, Niko},
title = {{F}irst experiments with ultrashort, circularly polarized
soft x-ray pulses at {FLASH}2},
journal = {Structural dynamics},
volume = {12},
number = {3},
issn = {2329-7778},
address = {Melville, NY},
publisher = {AIP Publishing LLC},
reportid = {PUBDB-2025-00512},
pages = {034301},
year = {2025},
note = {Additional grant:Deutsche Forschungsgemeinschaft (DFG) -
ProjectID 328545488 - TRR 227 “Ultrafast Spin
Dynamics”.},
abstract = {Time-resolved absorption Spectroscopy as well as Magnetic
Circular Dichroism with circularpolarized soft X-rays (XAS
and XMCD) are powerful tools to probe electronic and
magnetic dynamicsin magnetic materials in an element- and
site selective manner. Employing these
methods,groundbreaking results have been achieved for
instance for magnetic alloys, which helped to
fundamentallyadvance the field. The possibilities for
ultrafast XAS and XMCD experiments, haverecently improved:
In an upgrade of the free electron laser FLASH, a variable
polarization afterburnerundulator at FLASH2 was installed in
September 2023. This upgrade allows the generationof few
tens of femtosecond short circularly polarized soft X-ray
pulses covering the L2,3-edges of theimportant 3d transition
metal elements. Here, we present first experimental results
with circularlypolarized ultrashort X-ray pulses from the
FL23 beamline employing XMCD at the L-edges of the3d
elements, Co, Fe and Ni. We obtain significant XMCD, which
hints to a degree of circular polarizationclose to $100\%.$
Making use of the full pulse-length preserving monochromator
capabilitiesof FL23 and an improved pump laser setup, FLASH
offers important and efficient experimentalinfrastructure
for ultrafast spin dynamics studies in 3d transition
metals.},
cin = {DOOR ; HAS-User / FS-FLASH / FS-FLASH-B / FS-FLASH-O /
CFEL-XAC},
ddc = {500},
cid = {I:(DE-H253)HAS-User-20120731 / I:(DE-H253)FS-FLASH-20140814
/ I:(DE-H253)FS-FLASH-B-20160930 /
I:(DE-H253)FS-FLASH-O-20160930 /
I:(DE-H253)CFEL-XAC-20240710},
pnm = {631 - Matter – Dynamics, Mechanisms and Control
(POF4-631) / 6G2 - FLASH (DESY) (POF4-6G2) / FS-Proposal:
F-20211728 EC (F-20211728-EC) / FS-Proposal: F-20220710
(F-20220710) / DFG project G:(GEPRIS)328545488 - TRR 227:
Ultraschnelle Spindynamik (328545488)},
pid = {G:(DE-HGF)POF4-631 / G:(DE-HGF)POF4-6G2 /
G:(DE-H253)F-20211728-EC / G:(DE-H253)F-20220710 /
G:(GEPRIS)328545488},
experiment = {EXP:(DE-H253)F-PL23-20230101},
typ = {PUB:(DE-HGF)16},
pubmed = {40352094},
UT = {WOS:001488980600001},
doi = {10.1063/4.0000298},
url = {https://bib-pubdb1.desy.de/record/622831},
}