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@ARTICLE{Wenthaus:620104,
author = {Wenthaus, Lukas and Kabachnik, Nikolay and Borgwardt, Mario
and Palutke, Steffen and Kutnyakhov, Dmytro and Pressacco,
Federico and Scholz, Markus and Potorochin, Dmitrii and
Wind, Nils and Duesterer, Stefan and Brenner, Guenter and
Gessner, Oliver and Molodtsov, Serguei and Eberhardt,
Wolfgang and Roth, Friedrich},
title = {{I}nsights into the laser-assisted photoelectric effect
from solid-state surfaces},
reportid = {PUBDB-2025-00022, arXiv:2309.00099},
year = {2024},
note = {18 pages, 3 figures},
abstract = {Photoemission from a solid surface provides a wealth of
information about the electronic structure of the surface
and its dynamic evolution. Ultrafast pump-probe experiments
are particularly useful to study the dynamic interactions of
photons with surfaces as well as the ensuing electron
dynamics induced by these interactions. Time-resolved
laser-assisted photoemission (tr-LAPE) from surfaces is a
novel technique to gain deeper understanding of the
fundamentals underlying the photoemission process. Here, we
present the results of a femtosecond time-resolved soft
X-ray photoelectron spectroscopy experiment on two different
metal surfaces conducted at the X-ray Free-Electron Laser
FLASH in Hamburg. We study photoemission from the W 4f and
Pt 4f core levels using ultrashort soft X-ray pulses in
combination with synchronized infrared (IR) laser pulses.
When both pulses overlap in time and space, laser-assisted
photoemission results in the formation of a series of
sidebands that reflect the dynamics of the laser-surface
interaction. We demonstrate a qualitatively new level of
sideband generation up to the sixth order and a surprising
material dependence of the number of sidebands that has so
far not been predicted by theory. We provide a
semi-quantitative explanation of this phenomenon based on
the different dynamic dielectric responses of the two
materials. Our results advance the understanding of the LAPE
process and reveal new details of the IR field present in
the surface region, which is determined by the dynamic
interplay between the IR laser field and the dielectric
response of the metal surfaces.},
cin = {DOOR ; HAS-User / FS-LA / FS-FLASH-O / FS-FLASH /
FS-FLASH-B / $XFEL_E2_THE$ / $XFEL_DO_DD$ / FS-SXQM /
FS-PET-S},
ddc = {530},
cid = {I:(DE-H253)HAS-User-20120731 / I:(DE-H253)FS-LA-20130416 /
I:(DE-H253)FS-FLASH-O-20160930 /
I:(DE-H253)FS-FLASH-20140814 /
I:(DE-H253)FS-FLASH-B-20160930 /
$I:(DE-H253)XFEL_E2_THE-20210408$ /
$I:(DE-H253)XFEL_DO_DD-20210408$ /
I:(DE-H253)FS-SXQM-20190201 / I:(DE-H253)FS-PET-S-20190712},
pnm = {631 - Matter – Dynamics, Mechanisms and Control
(POF4-631) / 6G2 - FLASH (DESY) (POF4-6G2) / 05K22OF2 -
Untersuchungen des Ladungstransfers an Grenzflächen mittels
pikosekunden zeitaufgelöster Photoelektronenspektroskopie
bei Umgebungsdruck (BMBF-05K22OF2) / SFB 925 B02 -
Ultraschnelle Dynamik in stark korrelierten Systemen (B02)
(201270818)},
pid = {G:(DE-HGF)POF4-631 / G:(DE-HGF)POF4-6G2 /
G:(DE-Ds200)BMBF-05K22OF2 / G:(GEPRIS)201270818},
experiment = {EXP:(DE-H253)F-PG2-20150101},
typ = {PUB:(DE-HGF)25},
eprint = {2309.00099},
howpublished = {arXiv:2309.00099},
archivePrefix = {arXiv},
SLACcitation = {$\%\%CITATION$ = $arXiv:2309.00099;\%\%$},
url = {https://bib-pubdb1.desy.de/record/620104},
}