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@PHDTHESIS{Aufleger:619959,
author = {Aufleger, Lennart},
othercontributors = {Pfeifer, Thomas and Wolf, Andreas},
title = {{N}onlinear spectroscopy on an autoionizing two-electron
resonance in intense, extreme ultraviolet fields at a
free-electron laser},
school = {Heidelberg University},
type = {Dissertation},
publisher = {Heidelberg University Library},
reportid = {PUBDB-2024-08050},
pages = {119},
year = {2022},
note = {Dissertation, Heidelberg University, 2022},
abstract = {In this work, the influence of intense extreme-ultraviolet
(XUV) fields on helium is experimentally investigated.
Therefore, XUV pulses from a free-electron laser (FEL) are
combined with transient absorption spectroscopy (TAS) and
explored with numerical quantum-mechanical simulations. A
novel TAS beamline enables measurements on the prototypical
atomic three-body system, helium, at the free-electron laser
in Hamburg (FLASH). In particular, the energetically lowest
two-electron resonance, 2s2p, with its asymmetric Fano
absorption line shape is of interest. This bound state is
embedded in the single-ionization continuum and thus
represents an atomic interferometer. Its main property, the
sensitivity to phase, is used in this work to detect
manipulations induced by strong XUV pulses. In the
experiments, a distortion of the absorption line is observed
in the presence of highly intense XUV pulses. Firstly, the
line shape’s symmetry change is investigated with a
numerical few-level model simulation and found to be
connected to the transient dressing of the excited state.
Employing realistically modelled stochastic pulses, the
investigation is extended to the line shape’s dependence
on the pulse duration. Finally, the line broadening is
explained by the model simulation and allows for
disentangling the contributing mechanisms, two-photon
absorption and the increased reversion to the ground state.},
cin = {DOOR ; HAS-User},
cid = {I:(DE-H253)HAS-User-20120731},
pnm = {6G2 - FLASH (DESY) (POF4-6G2)},
pid = {G:(DE-HGF)POF4-6G2},
experiment = {EXP:(DE-H253)F-BL2-20150101},
typ = {PUB:(DE-HGF)11},
urn = {urn:nbn:de:bsz:16-heidok-312094},
url = {https://bib-pubdb1.desy.de/record/619959},
}