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@ARTICLE{Hoeppe:617635,
author = {Hoeppe, Hannes P and Osterhoff, Markus and Aghel Maleki,
Atiyeh and Rosselló, Juan M and Vassholz, Malte and
Hagemann, Johannes and Engler, Thea and Schwarz, Daniel and
Rodriguez-Fernandez, Angel and Boesenberg, Ulrike and
Möller, Johannes and Shayduk, Roman and Hallmann, Jörg and
Madsen, Anders and Mettin, Robert and Salditt, Tim},
title = {{T}he collapse of a sonoluminescent cavitation bubble
imaged with {X}-ray free-electron laser pulses},
journal = {New journal of physics},
volume = {26},
number = {3},
issn = {1367-2630},
address = {[London]},
publisher = {IOP},
reportid = {PUBDB-2024-06941},
pages = {033002},
year = {2024},
note = {DFG grant Me 1645/5-2.},
abstract = {Single bubble sonoluminescence (SBSL) is the phenomenon of
synchronous light emission due to the violent collapse of a
single spherical bubble in a liquid, driven by an ultrasonic
field. During the bubble collapse, matter inside the bubble
reaches extreme conditions of several gigapascals and
temperatures on the order of 10000 K, leading to
picosecond flashes of visible light. To this day, details
regarding the energy focusing mechanism rely on simulations
due to the fast dynamics of the bubble collapse and spatial
scales below the optical resolution limit. In this work we
present phase-contrast holographic imaging with single x-ray
free-electron laser (XFEL) pulses of a SBSL cavitation
bubble in water. X-rays probe the electron density structure
and by that provide a uniquely new view on the bubble
interior and its collapse dynamics. The involved fast
time-scales are accessed by sub-100 fs XFEL pulses and a
custom synchronization scheme for the bubble oscillator. We
find that during the whole oscillation cycle the bubble's
density profile can be well described by a simple step-like
structure, with the radius R following the dynamics of the
Gilmore model. The quantitatively measured internal density
and width of the boundary layer exhibit a large variance.
Smallest reconstructed bubble sizes reach down to R ≃ 0.8
μm, and are consistent with spherical symmetry. While we
here achieved a spatial resolution of a few 100 nm, the
visibility of the bubble and its internal structure is
limited by the total x-ray phase shift which can be scaled
with experimental parameters.},
cin = {FS-PETRA / $XFEL_E1_MID$},
ddc = {530},
cid = {I:(DE-H253)FS-PETRA-20140814 /
$I:(DE-H253)XFEL_E1_MID-20210408$},
pnm = {631 - Matter – Dynamics, Mechanisms and Control
(POF4-631) / HIDSS-0002 - DASHH: Data Science in Hamburg -
Helmholtz Graduate School for the Structure of Matter
$(2019_IVF-HIDSS-0002)$},
pid = {G:(DE-HGF)POF4-631 / $G:(DE-HGF)2019_IVF-HIDSS-0002$},
experiment = {EXP:(DE-H253)XFEL-SASE2-20150101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:001176689700001},
doi = {10.1088/1367-2630/ad295b},
url = {https://bib-pubdb1.desy.de/record/617635},
}