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@ARTICLE{Krieke:616642,
author = {Krieke, Guna and Antuzevics, Andris and Kalinko, Aleksandr
and Kuzmin, Aleksejs and Murauskas, Tomas and Kareiva,
Aivaras and Zarkov, Aleksej},
title = {{M}atrix-dependent high-contrast photochromism in
{E}u-doped {M}$_3${M}g{S}i$_2${O}$_8$ ({M} = {C}a, {S}r,
{B}a)},
journal = {The journal of physical chemistry / C},
volume = {12},
number = {41},
issn = {2050-7526},
address = {Washington, DC},
publisher = {Soc.},
reportid = {PUBDB-2024-06510},
pages = {16989-16998},
year = {2024},
abstract = {The photochromic properties and charge transfer processes
were studied in novel Eu-doped M$_3$MgSi$_2$O$_8$ (M = Ca,
Sr, Ba) compounds. These materials exhibit vivid color
changes upon irradiation with UV light, resulting in orange,
reddish-pink, and green colors. The introduction of europium
ions enhances photochromic efficiency and shifts excitation
peaks to lower energy ranges. Analysis of diffuse
reflectance and electron paramagnetic resonance spectra
reveals the formation of both paramagnetic and
non-paramagnetic defects, with the dominant signals
attributed to electron centers, likely F$^+$-type centers.
The Eu$^{2+}$ → Eu$^{3+}$ charge transfer during
irradiation indicates that Eu$^{2+}$ acts as a hole center.
These findings contribute to a better understanding of the
mechanisms underlying photochromism in these materials and
highlight their potential for practical applications.},
cin = {DOOR ; HAS-User},
ddc = {530},
cid = {I:(DE-H253)HAS-User-20120731},
pnm = {6G3 - PETRA III (DESY) (POF4-6G3) / FS-Proposal: I-20230821
EC (I-20230821-EC) / CAMART2 - Centre of Advanced Materials
Research and Technology Transfer CAMART² (739508)},
pid = {G:(DE-HGF)POF4-6G3 / G:(DE-H253)I-20230821-EC /
G:(EU-Grant)739508},
experiment = {EXP:(DE-H253)P-P64-20150101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:001317139200001},
doi = {10.1039/D4TC03091E},
url = {https://bib-pubdb1.desy.de/record/616642},
}