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@ARTICLE{Domrse:616009,
author = {Domröse, Till and Fernandez, Noelia and Eckel, Christian
and Rossnagel, Kai and Weitz, R. Thomas and Ropers, Claus},
title = {{N}anoscale {O}perando {I}maging of {E}lectrically {D}riven
{C}harge-{D}ensity {W}ave {P}hase {T}ransitions},
journal = {Nano letters},
volume = {24},
number = {40},
issn = {1530-6984},
address = {Washington, DC},
publisher = {ACS Publ.},
reportid = {PUBDB-2024-06305},
pages = {12476-12485},
year = {2024},
abstract = {Structural transformations in strongly correlated materials
promise efficient and fast control of materials’
properties via electrical or optical stimulation. The
desired functionality of devices operating based on phase
transitions, however, will also be influenced by nanoscale
heterogeneity. Experimentally characterizing the
relationship between microstructure and phase switching
remains challenging, as nanometer resolution and high
sensitivity to subtle structural modifications are required.
Here, we demonstrate nanoimaging of a current-induced phase
transformation in the charge-density wave (CDW) material
1T-TaS$_2$. Combining electrical characterizations with
tailored contrast enhancement, we correlate macroscopic
resistance changes with the nanoscale nucleation and growth
of CDW phase domains. In particular, we locally determine
the transformation barrier in the presence of dislocations
and strain, underlining their non-negligible impact on
future functional devices. Thereby, our results demonstrate
the merit of tailored contrast enhancement and beam shaping
for advanced operando microscopy of quantum materials and
devices.},
cin = {FS-SXQM},
ddc = {660},
cid = {I:(DE-H253)FS-SXQM-20190201},
pnm = {632 - Materials – Quantum, Complex and Functional
Materials (POF4-632) / SFB 1073 A05 - Nanoskalige
Untersuchung raumzeitlicher Relaxation in heterogenen
Systemen (A05) (240159667) / DFG project G:(GEPRIS)217133147
- SFB 1073: Kontrolle von Energiewandlung auf atomaren
Skalen (217133147)},
pid = {G:(DE-HGF)POF4-632 / G:(GEPRIS)240159667 /
G:(GEPRIS)217133147},
experiment = {EXP:(DE-MLZ)NOSPEC-20140101},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:39316412},
UT = {WOS:001319875400001},
doi = {10.1021/acs.nanolett.4c03324},
url = {https://bib-pubdb1.desy.de/record/616009},
}