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000615828 1001_ $$0P:(DE-H253)PIP1091707$$aLuo, Cheng$$b0
000615828 245__ $$aSpectral fingerprinting of aqueous glucose with ultra-broadband vibrational sum-frequency generation spectroscopy at bio-relevant low concentration
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000615828 520__ $$aVibrational modes of glucose spanning from 900 to 1400 cm$^{−1}$ in the molecular fingerprint region have been traced by means of vibrational sum-frequency generation spectroscopy in aqueous solution as a function of glucose concentration. The high sensitivity is enabled by a 200 kHz few-cycle mid-infrared optical parametric chirped-pulse amplifier (OPCPA). The OPCPA generates broadband pulses (from 7 to 11 µm) centered at 9 µm with 114 fs pulse duration, at a high average power of 245 mW and high pulse energy of 1.2 µJ. The achieved performance of the spectrometer is benchmarked by probing the carbon-oxygen bond stretching mode at 1035 cm using a biologically relevant low sample concentration of 10 mM.
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000615828 7001_ $$0P:(DE-H253)PIP1083742$$aVasudevan Namboodiri, Mahesh$$b1
000615828 7001_ $$0P:(DE-HGF)0$$aSchulz, Michael$$b2
000615828 7001_ $$0P:(DE-HGF)0$$aRiedel, Robert$$b3
000615828 7001_ $$0P:(DE-H253)PIP1015357$$aPrandolini, Mark$$b4
000615828 7001_ $$0P:(DE-H253)PIP1006367$$aLaarmann, Tim$$b5$$eCorresponding author
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