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000615688 037__ $$aPUBDB-2024-06252
000615688 041__ $$aEnglish
000615688 1001_ $$0P:(DE-H253)PIP1025162$$aLindenblatt, Hannes$$b0$$eCorresponding author$$gmale
000615688 245__ $$aEnergy and Charge Transfer in Dimers and Trimers of Xenon$$f2020-11-08 - 2023-11-08
000615688 260__ $$bHeidelberg University Library$$c2023
000615688 300__ $$a149
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000615688 502__ $$aDissertation, Heidelberg University, 2023$$bDissertation$$cHeidelberg University$$d2023$$o2023-11-08
000615688 520__ $$aThe goal of this thesis is the investigation of decay processes in innershell ionised xenon dimers and trimers. To this end, the small clusters were ionised using 100 eV photons from a Free-Electron Laser and the momenta of the created ion fragments and electrons were measured using the Reaction Microscope at FLASH2. Employing an XUV/XUV pump-probe scheme, the timescale to distribute energy or charge throughout the cluster following local excitation was determined to below (186+-6) fs for dimers decaying into Xe$^{1+}$ / Xe$^{2+}$ and (84+-13) fs for trimers decaying into Xe$^{1+}/Xe^{1+}/Xe^{1+}$. The kinetic energy distributions yield clear evidence that Xe$_2^{2+}$ decays by a slow CT process after bond contraction and Xe$_3^{2+*}$ decays by ETMD(3) before the nuclei can move. Furthermore, we see signatures of frustrated ionisation in Xe$_2$ dimers. 
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000615688 650_7 $$2Other$$a530 Physics
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000615688 7001_ $$0P:(DE-H253)PIP1007317$$aMoshammer, Robert$$b1$$eThesis advisor
000615688 7001_ $$0P:(DE-HGF)0$$aQuint, Wolfgang$$b2$$eThesis advisor
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