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@ARTICLE{Garain:615365,
author = {Garain, Swadhin and Li, Pei-Lun and Shoyama, Kazutaka and
Wuerthner, Frank},
title = {2,3 : 6,7‐{N}aphthalene {B}is(dicarboximide)
{C}yclophane: {A} {P}hotofunctional {H}ost for {A}mbient
{D}elayed {F}luorescence in {S}olution},
journal = {Angewandte Chemie / International edition},
volume = {63},
number = {43},
issn = {1433-7851},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {PUBDB-2024-06120},
pages = {e202411102},
year = {2024},
abstract = {Harvesting triplet excitons of heavy atom-free purely
organic chromophores under aerated conditions is challenging
due to the quenching of long-lived triplet states by
molecular oxygen and vibrational dissipation. Herein, we
show a supramolecular approach of triplet harvesting via
mitigating quenching pathways of a triplet harvester.
Specifically, we used a host–guest system based on
2,3 : 6,7-naphthalene bis(dicarboximide)-derived
cyclophane (NBICy) and carbazole derivative (EtCz).
Complexation studies and single-crystal X-ray analysis
showed the formation of a rigid host–guest complex
(K≈10$^4$ M$^{−1}$ in CCl$_4$), resulting in
triplet-exciton stabilization under aerated conditions via
mitigating vibrational interference and oxygen quenching.
Photophysical studies elucidate the delayed fluorescence
emission from the charge-transfer state (1CT) with a quantum
yield (QY) of 6–8 \% under ambient conditions which
increased up to 36 \% in an inert atmosphere.},
cin = {DOOR ; HAS-User},
ddc = {540},
cid = {I:(DE-H253)HAS-User-20120731},
pnm = {6G3 - PETRA III (DESY) (POF4-6G3) / FS-Proposal: I-20231007
(I-20231007)},
pid = {G:(DE-HGF)POF4-6G3 / G:(DE-H253)I-20231007},
experiment = {EXP:(DE-H253)P-P11-20150101},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:39003722},
UT = {WOS:001341180800014},
doi = {10.1002/anie.202411102},
url = {https://bib-pubdb1.desy.de/record/615365},
}