000614119 001__ 614119 000614119 005__ 20250723172345.0 000614119 0247_ $$2doi$$a10.1021/jacs.3c12883 000614119 0247_ $$2ISSN$$a0002-7863 000614119 0247_ $$2ISSN$$a1520-5126 000614119 0247_ $$2ISSN$$a1943-2984 000614119 0247_ $$2datacite_doi$$a10.3204/PUBDB-2024-05753 000614119 0247_ $$2altmetric$$aaltmetric:164391745 000614119 0247_ $$2pmid$$apmid:38848551 000614119 0247_ $$2WOS$$aWOS:001242732500001 000614119 0247_ $$2openalex$$aopenalex:W4399420574 000614119 037__ $$aPUBDB-2024-05753 000614119 041__ $$aEnglish 000614119 082__ $$a540 000614119 1001_ $$aBaxter, James M.$$b0 000614119 245__ $$aPower Density Titration of Reversible Photoisomerization of a Fluorescent Protein Chromophore in the Presence of Thermally Driven Barrier Crossing Shown by Quantitative Millisecond Serial Synchrotron X-ray Crystallography 000614119 260__ $$aWashington, DC$$bACS Publications$$c2024 000614119 3367_ $$2DRIVER$$aarticle 000614119 3367_ $$2DataCite$$aOutput Types/Journal article 000614119 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1725966910_1898298 000614119 3367_ $$2BibTeX$$aARTICLE 000614119 3367_ $$2ORCID$$aJOURNAL_ARTICLE 000614119 3367_ $$00$$2EndNote$$aJournal Article 000614119 520__ $$aWe present millisecond quantitative serial X-ray crystallography at 1.7 Å resolution demonstrating precise optical control of reversible population transfer from Trans–Cis and Cis–Trans photoisomerization of a reversibly switchable fluorescent protein, rsKiiro. Quantitative results from the analysis of electron density differences, extrapolated structure factors, and occupancy refinements are shown to correspond to optical measurements of photoinduced population transfer and have sensitivity to a few percent in concentration differences. Millisecond time-resolved concentration differences are precisely and reversibly controlled through intense continuous wave laser illuminations at 405 and 473 nm for the Trans-to-Cis and Cis-to-Trans reactions, respectively, while the X-ray crystallographic measurement and laser illumination of the metastable Trans chromophore conformation causes partial thermally driven reconversion across a 91.5 kJ/mol thermal barrier from which a temperature jump between 112 and 128 K is extracted. 000614119 536__ $$0G:(DE-HGF)POF4-6G3$$a6G3 - PETRA III (DESY) (POF4-6G3)$$cPOF4-6G3$$fPOF IV$$x0 000614119 536__ $$0G:(GEPRIS)390715994$$aDFG project 390715994 - EXC 2056: CUI: Advanced Imaging of Matter (390715994)$$c390715994$$x1 000614119 536__ $$0G:(GEPRIS)194651731$$aDFG project 194651731 - EXC 1074: Hamburger Zentrum für ultraschnelle Beobachtung (CUI): Struktur, Dynamik und Kontrolle von Materie auf atomarer Skala (194651731)$$c194651731$$x2 000614119 536__ $$0G:(GEPRIS)390540038$$aDFG project 390540038 - EXC 2008: Unifying Systems in Catalysis "UniSysCat" (390540038)$$c390540038$$x3 000614119 542__ $$2Crossref$$i2024-06-07$$uhttps://creativecommons.org/licenses/by/4.0/ 000614119 588__ $$aDataset connected to CrossRef, Journals: bib-pubdb1.desy.de 000614119 693__ $$0EXP:(DE-H253)P-P14-20150101$$1EXP:(DE-H253)PETRAIII-20150101$$6EXP:(DE-H253)P-P14-20150101$$aPETRA III$$fPETRA Beamline P14$$x0 000614119 693__ $$0EXP:(DE-H253)P-P11-20150101$$1EXP:(DE-H253)PETRAIII-20150101$$6EXP:(DE-H253)P-P11-20150101$$aPETRA III$$fPETRA Beamline P11$$x1 000614119 7001_ $$aHutchison, Christopher D. M.$$b1 000614119 7001_ $$aFadini, Alisia$$b2 000614119 7001_ $$aMaghlaoui, Karim$$b3 000614119 7001_ $$aCordon-Preciado, Violeta$$b4 000614119 7001_ $$aMorgan, R. Marc L.$$b5 000614119 7001_ $$0P:(DE-H253)PIP1026545$$aAgthe, Michael$$b6 000614119 7001_ $$aHorrell, Sam$$b7 000614119 7001_ $$aTellkamp, Friedjof$$b8 000614119 7001_ $$0P:(DE-H253)PIP1029103$$aMehrabi, Pedram$$b9 000614119 7001_ $$aPfeifer, Yannik$$b10 000614119 7001_ $$0P:(DE-HGF)0$$aMüller-Werkmeister, Henrike M.$$b11 000614119 7001_ $$0P:(DE-HGF)0$$avon Stetten, David$$b12 000614119 7001_ $$aPearson, Arwen R.$$b13 000614119 7001_ $$0P:(DE-HGF)0$$avan Thor, Jasper J.$$b14$$eCorresponding author 000614119 77318 $$2Crossref$$3journal-article$$a10.1021/jacs.3c12883$$bAmerican Chemical Society (ACS)$$d2024-06-07$$n24$$p16394-16403$$tJournal of the American Chemical Society$$v146$$x0002-7863$$y2024 000614119 773__ $$0PERI:(DE-600)1472210-0$$a10.1021/jacs.3c12883$$gVol. 146, no. 24, p. 16394 - 16403$$n24$$p16394-16403$$tJournal of the American Chemical Society$$v146$$x0002-7863$$y2024 000614119 8564_ $$uhttps://pubs.acs.org/doi/10.1021/jacs.3c12883 000614119 8564_ 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