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@ARTICLE{Kwiatkowksi:614022,
author = {Kwiatkowksi, Anna and Caserta, Giorgio and Schulz,
Anne-Christine and Frielingsdorf, Stefan and Pelmenschikov,
Vladimir and Weisser, Kilian and Belsom, Adam and
Rappsilber, Juri and Sergeev, Ilya and Limberg, Christian
and Mroginski, Maria-Andrea and Zebger, Ingo and Lenz,
Oliver},
title = {{ATP}-triggered {F}e({CN})$_2${CO} synthon transfer from
the maturase {H}yp{CD} to the active site of
apo-[{N}i{F}e]-hydrogenase},
reportid = {PUBDB-2024-05723},
year = {2024},
note = {Funding: Deutsche Forschungsgemeinschaft (DFG, German
Research Foundation) through SPP 1927 “Iron Sulfur for
Life” project no 311062227; the cluster of excellence
‘UniSysCat’ under Germany’s Excellence
Strategy-EXC2008-390540038. EU: the COST Action
FeSImmChemNet, CA21115, supported by COST (European
Cooperation in Science and Technology).},
abstract = {[NiFe]-hydrogenases catalyze the reversible activation of
H$_2$ using a unique NiFe(CN)$_2$CO metal site, which is
assembled by a sophisticated multi-protein machinery. The
[4Fe–4S]-cluster-containing HypCD complex, which possesses
an ATPase activity with an hitherto unknown function, serves
as the hub for the assembly of the Fe(CN)$_2$CO
sub-fragment. HypCD is also thought to be responsible for
the subsequent transfer of the iron fragment to the apo-form
of the catalytic hydrogenase subunit, but the underlying
mechanism remained unexplored. Here, we performed a thorough
spectroscopic characterization of different HypCD
preparations using infrared, Mössbauer and NRVS
spectroscopy, revealing molecular details of the
coordination of the Fe(CN)$_2$CO fragment. Moreover,
biochemical assays in combination with spectroscopy,
AlphaFold structure predictions, protein-ligand docking
calculations and crosslinking MS deciphered unexpected
mechanistic aspects of the ATP requirement of HypCD, which
we found to actually trigger the transfer of the
Fe(CN)$_2$CO fragment to the apo-hydrogenase.},
cin = {DOOR ; HAS-User / FS-PET-S},
cid = {I:(DE-H253)HAS-User-20120731 /
I:(DE-H253)FS-PET-S-20190712},
pnm = {632 - Materials – Quantum, Complex and Functional
Materials (POF4-632) / 6G3 - PETRA III (DESY) (POF4-6G3) /
FS-Proposal: I-20220851 (I-20220851) / FS-Proposal:
I-20210325 (I-20210325) / DFG project G:(GEPRIS)311062227 -
Die Rolle von Eisen-Schwefel-Kofaktoren in der Assemblierung
von Metallzentren und der Katalyse von Hydrogenasen
(311062227) / DFG project G:(GEPRIS)449713269 - Design,
Synthese und Analyse von photospaltbaren chemischen
Crosslinkern zur Entwicklung von verbesserten Methoden in
der Crosslinking Massenspektrometrie (449713269)},
pid = {G:(DE-HGF)POF4-632 / G:(DE-HGF)POF4-6G3 /
G:(DE-H253)I-20220851 / G:(DE-H253)I-20210325 /
G:(GEPRIS)311062227 / G:(GEPRIS)449713269},
experiment = {EXP:(DE-H253)P-P01-20150101},
typ = {PUB:(DE-HGF)25},
doi = {10.26434/chemrxiv-2024-3dx2g},
url = {https://bib-pubdb1.desy.de/record/614022},
}