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| Home > Publications database > Self-Stacked 1T-1H Layers in 6R-NbSeTe and the Emergence of Charge and Magnetic Correlations Due to Ligand Disorder > print |
| 001 | 613732 | ||
| 005 | 20250715171140.0 | ||
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| 100 | 1 | _ | |a Mahatha, Sanjoy Kr |0 P:(DE-H253)PIP1085751 |b 0 |
| 245 | _ | _ | |a Self-Stacked 1T-1H Layers in 6R-NbSeTe and the Emergence of Charge and Magnetic Correlations Due to Ligand Disorder |
| 260 | _ | _ | |a Washington, DC |c 2024 |b Soc. |
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| 520 | _ | _ | |a The emergence of correlated phenomena arising from the combination of 1T and 1H van der Waals layers is the focus of intense research. Here, we synthesize a self-stacked 6R phase in NbSeTe, showing perfect alternating 1T and 1H layers that grow coherently along the c-direction, as revealed by scanning transmission electron microscopy. Angle-resolved photoemission spectroscopy shows a mixed contribution of the trigonal and octahedral Nb bands to the Fermi level. Diffuse scattering reveals temperature-independent short-range charge fluctuations with propagation vector qCO = (0.25 0), derived from the condensation of a longitudinal mode in the 1T layer, while the long-range charge density wave is quenched by ligand disorder. Magnetization measurements suggest the presence of an inhomogeneous, short-range magnetic order, further supported by the absence of a clear phase transition in the specific heat. These experimental analyses in combination with ab initio calculations indicate that the ground state of 6R-NbSeTe is described by a statistical distribution of short-range charge-modulated and spin-correlated regions driven by ligand disorder. Our results demonstrate how natural 1T-1H self-stacked bulk heterostructures can be used to engineer emergent phases of matter. |
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| 700 | 1 | _ | |a Phillips, Jan |b 1 |
| 700 | 1 | _ | |a Corral-Sertal, Javier |b 2 |
| 700 | 1 | _ | |a Subires, David |b 3 |
| 700 | 1 | _ | |a Korshunov, Artem |b 4 |
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| 700 | 1 | _ | |a Fumega, Adolfo O. |0 0000-0002-3385-6409 |b 16 |
| 700 | 1 | _ | |a Blanco-Canosa, Santiago |0 P:(DE-H253)PIP1033306 |b 17 |e Corresponding author |
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| 856 | 4 | _ | |y Published on 2024-08-01. Available in OpenAccess from 2025-08-01. |u https://bib-pubdb1.desy.de/record/613732/files/document.pdf |
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