000612725 001__ 612725
000612725 005__ 20240913212701.0
000612725 037__ $$aPUBDB-2024-05442
000612725 041__ $$aEnglish
000612725 1001_ $$0P:(DE-H253)PIP1012175$$aKüpper, Jochen$$b0$$eCorresponding author$$udesy
000612725 1112_ $$a17th Quantum Reactive Scattering Workshop$$cIstanbul$$d2024-06-24 - 2024-06-28$$gQRS 2024$$wTurkey
000612725 245__ $$aDynamics of microsolvated (bio)molecules
000612725 260__ $$c2024
000612725 3367_ $$033$$2EndNote$$aConference Paper
000612725 3367_ $$2DataCite$$aOther
000612725 3367_ $$2BibTeX$$aINPROCEEDINGS
000612725 3367_ $$2DRIVER$$aconferenceObject
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000612725 3367_ $$0PUB:(DE-HGF)6$$2PUB:(DE-HGF)$$aConference Presentation$$bconf$$mconf$$s1726234630_4150639$$xInvited
000612725 520__ $$aObserving molecules in action through the recording of 'molecular movies', i.e., their spatiotemporal evolution during chemical dynamics, with atomic spatial and temporal resolution promises to revolutionize our understanding of the molecular sciences and to provide a time-dependent basis of chemistry. Experimentally, we build upon our approaches to prepare highly controlled samples that enable advanced imaging methods of individual molecular species directly in the molecular frame. We prepare highly controlled molecular samples for advanced ultrafast imaging experiments. This includes the preparation of ensembles of individual molecular species, e.g., single microsolvation environments, single conformers, or even single quantum states. Furthermore, the generated very cold samples are ideally suited to fix the molecules in space in laser-alignment or mixed-field orientation approaches. Here, we used the electric deflector to spatially separate different molecular species in combination with pump-probe velocity-map-imaging experiments, including utilization of 4D 'cameras'. We demonstrated that this powerful experimental approach reveals intimate details, e.g., on the radiation damage and fragmentation of water-water and pyrrole-water dimers as well as on the UV-induced dynamics in the near-UV-absorbing prototypical biomolecular indole-water system. We determined the time-dependent appearance of the different reaction products and disentangled the occurring ultrafast processes. This novel approach ensures that the reactants are well-known and that detailed characteristics of the specific reaction products are accessible – moving further toward the complete chemical-reactivity experiment.
000612725 536__ $$0G:(DE-HGF)POF4-631$$a631 - Matter – Dynamics, Mechanisms and Control (POF4-631)$$cPOF4-631$$fPOF IV$$x0
000612725 536__ $$0G:(GEPRIS)390715994$$aDFG project 390715994 - EXC 2056: CUI: Advanced Imaging of Matter (390715994)$$c390715994$$x1
000612725 693__ $$0EXP:(DE-H253)CFEL-Exp-20150101$$5EXP:(DE-H253)CFEL-Exp-20150101$$eExperiments at CFEL$$x0
000612725 8564_ $$uhttps://www.qrs17.ch/
000612725 909CO $$ooai:bib-pubdb1.desy.de:612725$$pVDB
000612725 9101_ $$0I:(DE-588b)2008985-5$$6P:(DE-H253)PIP1012175$$aDeutsches Elektronen-Synchrotron$$b0$$kDESY
000612725 9101_ $$0I:(DE-H253)_CFEL-20120731$$6P:(DE-H253)PIP1012175$$aCentre for Free-Electron Laser Science$$b0$$kCFEL
000612725 9101_ $$0I:(DE-588)1043621512$$6P:(DE-H253)PIP1012175$$aEuropean XFEL$$b0$$kXFEL.EU
000612725 9131_ $$0G:(DE-HGF)POF4-631$$1G:(DE-HGF)POF4-630$$2G:(DE-HGF)POF4-600$$3G:(DE-HGF)POF4$$4G:(DE-HGF)POF$$aDE-HGF$$bForschungsbereich Materie$$lVon Materie zu Materialien und Leben$$vMatter – Dynamics, Mechanisms and Control$$x0
000612725 9141_ $$y2024
000612725 9201_ $$0I:(DE-H253)FS-CFEL-CMI-20220405$$kFS-CFEL-CMI$$lCFEL-CMI$$x0
000612725 9201_ $$0I:(DE-H253)UNI_CUI-20121230$$kUNI/CUI$$lbeauftragt von UNI$$x1
000612725 9201_ $$0I:(DE-H253)UNI_EXP-20120731$$kUNI/EXP$$lUni Hamburg / Experimentalphysik$$x2
000612725 980__ $$aconf
000612725 980__ $$aVDB
000612725 980__ $$aI:(DE-H253)FS-CFEL-CMI-20220405
000612725 980__ $$aI:(DE-H253)UNI_CUI-20121230
000612725 980__ $$aI:(DE-H253)UNI_EXP-20120731
000612725 980__ $$aUNRESTRICTED