000611720 001__ 611720 000611720 005__ 20250723171923.0 000611720 0247_ $$2doi$$a10.1039/D4SC02907K 000611720 0247_ $$2ISSN$$a2041-6520 000611720 0247_ $$2ISSN$$a2041-6539 000611720 0247_ $$2datacite_doi$$a10.3204/PUBDB-2024-05033 000611720 0247_ $$2altmetric$$aaltmetric:165289400 000611720 0247_ $$2pmid$$apmid:39118611 000611720 0247_ $$2WOS$$aWOS:001275391000001 000611720 0247_ $$2openalex$$aopenalex:W4400503183 000611720 037__ $$aPUBDB-2024-05033 000611720 041__ $$aEnglish 000611720 082__ $$a540 000611720 1001_ $$0P:(DE-H253)PIP1094186$$aSarma, Bidyut Bikash$$b0$$eCorresponding author 000611720 245__ $$aUnderstanding the role of supported Rh atoms and clusters during hydroformylation and CO hydrogenation reactions with in situ / operando XAS and DRIFT spectroscopy 000611720 260__ $$aCambridge$$bRSC$$c2024 000611720 3367_ $$2DRIVER$$aarticle 000611720 3367_ $$2DataCite$$aOutput Types/Journal article 000611720 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1728892478_4011022 000611720 3367_ $$2BibTeX$$aARTICLE 000611720 3367_ $$2ORCID$$aJOURNAL_ARTICLE 000611720 3367_ $$00$$2EndNote$$aJournal Article 000611720 520__ $$aSupported Rh single-atoms and clusters on CeO2, MgO, and ZrO2 were investigated as catalysts for hydroformylation of ethylene to propionaldehyde and CO hydrogenation to methanol/ethanol with in situ/operando diffuse reflectance infrared Fourier transform spectroscopy (DRIFTS) and X-ray absorption spectroscopy (XAS). Under hydroformylation reaction conditions, operando spectroscopic investigations unravel the presence of both single atoms and clusters and detected at first propanal and then methanol. We find that the formation of methanol is associated with CO hydrogenation over Rh clusters which was further confirmed under CO hydrogenation conditions at elevated pressure. The activity of catalysts synthesized via a precipitation (PP) method over various supports towards the hydroformylation reaction follows the order: Rh/ZrO2 > Rh/CeO2 > Rh/MgO. Comparing Rh/CeO2 catalysts synthesized via different methods, catalysts prepared by flame spray pyrolysis (FSP) showed catalytic activity for the hydroformylation reaction at lower temperatures (413 K), whereas catalysts prepared by wet impregnation (WI) showed the highest stability. These results not only provide fundamental insights into the atomistic level of industrially relevant reactions but also pave the way for a rational design of new catalysts in the future. 000611720 536__ $$0G:(DE-HGF)POF4-6G3$$a6G3 - PETRA III (DESY) (POF4-6G3)$$cPOF4-6G3$$fPOF IV$$x0 000611720 536__ $$0G:(DE-H253)I-20200891$$aFS-Proposal: I-20200891 (I-20200891)$$cI-20200891$$x1 000611720 536__ $$0G:(DE-H253)I-20211473$$aFS-Proposal: I-20211473 (I-20211473)$$cI-20211473$$x2 000611720 536__ $$0G:(GEPRIS)446701131$$aSFB 1441 B03 - In situ/operando-Charakterisierung von Edelmetallclustern und Partikeln auf Metalloxiden unter Reaktionsbedingungen (B03) (446701131)$$c446701131$$x3 000611720 542__ $$2Crossref$$i2024-07-10$$uhttp://creativecommons.org/licenses/by-nc/3.0/ 000611720 588__ $$aDataset connected to CrossRef, Journals: bib-pubdb1.desy.de 000611720 693__ $$0EXP:(DE-H253)P-P65-20150101$$1EXP:(DE-H253)PETRAIII-20150101$$6EXP:(DE-H253)P-P65-20150101$$aPETRA III$$fPETRA Beamline P65$$x0 000611720 7001_ $$0P:(DE-H253)PIP1094188$$aNeukum, Dominik$$b1 000611720 7001_ $$0P:(DE-H253)PIP1017208$$aDoronkin, Dmitry$$b2 000611720 7001_ $$00009-0006-1680-3571$$aLakshmi Nilayam, Ajai Raj$$b3 000611720 7001_ $$0P:(DE-H253)PIP1100120$$aBaumgarten, Lorena$$b4 000611720 7001_ $$0P:(DE-H253)PIP1019792$$aKrause, Baerbel$$b5 000611720 7001_ $$0P:(DE-H253)PIP1008522$$aGrunwaldt, Jan-Dierk$$b6 000611720 77318 $$2Crossref$$3journal-article$$a10.1039/d4sc02907k$$bRoyal Society of Chemistry (RSC)$$d2024-01-01$$n31$$p12369-12379$$tChemical Science$$v15$$x2041-6520$$y2024 000611720 773__ $$0PERI:(DE-600)2559110-1$$a10.1039/D4SC02907K$$gp. 10.1039.D4SC02907K$$n31$$p12369-12379$$tChemical science$$v15$$x2041-6520$$y2024 000611720 8564_ $$uhttps://bib-pubdb1.desy.de/record/611720/files/d4sc02907k.pdf$$yOpenAccess 000611720 8564_ $$uhttps://bib-pubdb1.desy.de/record/611720/files/d4sc02907k.pdf?subformat=pdfa$$xpdfa$$yOpenAccess 000611720 909CO $$ooai:bib-pubdb1.desy.de:611720$$pdnbdelivery$$pdriver$$pVDB$$popen_access$$popenaire 000611720 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1094186$$aExternal Institute$$b0$$kExtern 000611720 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1094188$$aExternal Institute$$b1$$kExtern 000611720 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1017208$$aExternal Institute$$b2$$kExtern 000611720 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1100120$$aExternal Institute$$b4$$kExtern 000611720 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1019792$$aExternal Institute$$b5$$kExtern 000611720 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1008522$$aExternal Institute$$b6$$kExtern 000611720 9131_ $$0G:(DE-HGF)POF4-6G3$$1G:(DE-HGF)POF4-6G0$$2G:(DE-HGF)POF4-600$$3G:(DE-HGF)POF4$$4G:(DE-HGF)POF$$aDE-HGF$$bForschungsbereich Materie$$lGroßgeräte: Materie$$vPETRA III (DESY)$$x0 000611720 9141_ $$y2024 000611720 915__ $$0StatID:(DE-HGF)0160$$2StatID$$aDBCoverage$$bEssential Science Indicators$$d2023-10-26 000611720 915__ $$0LIC:(DE-HGF)CCBYNC4$$2HGFVOC$$aCreative Commons Attribution-NonCommercial CC BY-NC 4.0 000611720 915__ $$0StatID:(DE-HGF)1200$$2StatID$$aDBCoverage$$bChemical Reactions$$d2023-10-26 000611720 915__ $$0StatID:(DE-HGF)1210$$2StatID$$aDBCoverage$$bIndex Chemicus$$d2023-10-26 000611720 915__ $$0StatID:(DE-HGF)0113$$2StatID$$aWoS$$bScience Citation Index Expanded$$d2023-10-26 000611720 915__ $$0StatID:(DE-HGF)0510$$2StatID$$aOpenAccess 000611720 915__ $$0StatID:(DE-HGF)0430$$2StatID$$aNational-Konsortium$$d2024-12-13$$wger 000611720 915__ $$0StatID:(DE-HGF)0100$$2StatID$$aJCR$$bCHEM SCI : 2022$$d2024-12-13 000611720 915__ $$0StatID:(DE-HGF)0200$$2StatID$$aDBCoverage$$bSCOPUS$$d2024-12-13 000611720 915__ $$0StatID:(DE-HGF)0300$$2StatID$$aDBCoverage$$bMedline$$d2024-12-13 000611720 915__ $$0StatID:(DE-HGF)0199$$2StatID$$aDBCoverage$$bClarivate Analytics Master Journal List$$d2024-12-13 000611720 915__ $$0StatID:(DE-HGF)1150$$2StatID$$aDBCoverage$$bCurrent Contents - Physical, Chemical and Earth Sciences$$d2024-12-13 000611720 915__ $$0StatID:(DE-HGF)0150$$2StatID$$aDBCoverage$$bWeb of Science Core Collection$$d2024-12-13 000611720 915__ $$0StatID:(DE-HGF)0501$$2StatID$$aDBCoverage$$bDOAJ Seal$$d2024-07-23T09:28:57Z 000611720 915__ $$0StatID:(DE-HGF)0500$$2StatID$$aDBCoverage$$bDOAJ$$d2024-07-23T09:28:57Z 000611720 915__ $$0StatID:(DE-HGF)0030$$2StatID$$aPeer Review$$bDOAJ : Anonymous peer review$$d2024-07-23T09:28:57Z 000611720 915__ $$0StatID:(DE-HGF)9905$$2StatID$$aIF >= 5$$bCHEM SCI : 2022$$d2024-12-13 000611720 9201_ $$0I:(DE-H253)HAS-User-20120731$$kDOOR ; HAS-User$$lDOOR-User$$x0 000611720 980__ $$ajournal 000611720 980__ $$aVDB 000611720 980__ $$aUNRESTRICTED 000611720 980__ $$aI:(DE-H253)HAS-User-20120731 000611720 9801_ $$aFullTexts 000611720 999C5 $$1Franke$$2Crossref$$9-- missing cx lookup --$$a10.1021/cr3001803$$p5675 -$$tChem. 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