% IMPORTANT: The following is UTF-8 encoded. This means that in the presence % of non-ASCII characters, it will not work with BibTeX 0.99 or older. % Instead, you should use an up-to-date BibTeX implementation like “bibtex8” or % “biber”. @ARTICLE{Yachmenev:611712, author = {Yachmenev, Andrey and Onvlee, Jolijn and Zak, Emil and Owens, Alec and Küpper, Jochen}, title = {{F}ield-{I}nduced {D}iastereomers for {C}hiral {S}eparation}, reportid = {PUBDB-2024-05026, arXiv:1905.07166}, year = {2019}, abstract = {A novel approach for the state-specific enantiomeric enrichment and the spatial separation of enantiomers is presented. Our scheme utilizes techniques from strong-field laser physics, specifically an optical centrifuge in conjunction with a static electric field, to create a chiral field with defined handedness. Molecular enantiomers experience unique rotational excitation dynamics and this can be exploited to spatially separate the enantiomers using electrostatic deflection. Notably, the rotational-state-specific enantiomeric enhancement and its handedness is fully controllable. To explain these effects, we introduce the conceptual framework of $field\text{-}induced~diastereomers$ of a chiral molecule and perform robust quantum mechanical simulations on the prototypical chiral molecule propylene oxide (C$_3$H$_6$O), for which ensembles with an enantiomeric excess of up to $30~\\%$ were obtained.}, cin = {FS-CFEL-CMI / UNI/CUI / UNI/EXP}, ddc = {530}, cid = {I:(DE-H253)FS-CFEL-CMI-20220405 / $I:(DE-H253)UNI_CUI-20121230$ / $I:(DE-H253)UNI_EXP-20120731$}, pnm = {631 - Matter – Dynamics, Mechanisms and Control (POF4-631) / Ex-Net-0002-Phase2-3 - Advanced Imaging of Matter: Structure, Dynamics and Control on the Atomic Scale - AIM $(2018_Ex-Net-0002-Phase2-3)$ / COMOTION - Controlling the Motion of Complex Molecules and Particles (614507) / DFG project 281310165 - Abbildung chemischer Dynamik mittels laserinduzierter Elektronenbeugung im Molekülkoordinatensystem (281310165) / DFG project 390715994 - EXC 2056: CUI: Advanced Imaging of Matter (390715994) / DFG project 194651731 - EXC 1074: Hamburger Zentrum für ultraschnelle Beobachtung (CUI): Struktur, Dynamik und Kontrolle von Materie auf atomarer Skala (194651731)}, pid = {G:(DE-HGF)POF4-631 / $G:(DE-HGF)2018_Ex-Net-0002-Phase2-3$ / G:(EU-Grant)614507 / G:(GEPRIS)281310165 / G:(GEPRIS)390715994 / G:(GEPRIS)194651731}, experiment = {EXP:(DE-MLZ)NOSPEC-20140101}, typ = {PUB:(DE-HGF)25}, eprint = {1905.07166}, howpublished = {arXiv:1905.07166}, archivePrefix = {arXiv}, SLACcitation = {$\%\%CITATION$ = $arXiv:1905.07166;\%\%$}, pubmed = {pmid:31922822}, url = {https://bib-pubdb1.desy.de/record/611712}, }