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@ARTICLE{Zhang:607686,
      author       = {Zhang, Jichao and Zhu, Jiexin and Kang, Liqun and Zhang,
                      Qing and Liu, Longxiang and Guo, Fei and Li, Kaiqi and Feng,
                      Jianrui and Xia, Lixue and Lv, Lei and Zong, Wei and
                      Shearing, Paul R. and Brett, Dan J. L. and Parkin, Ivan P.
                      and Song, Xuedan and Mai, Liqiang and He, Guanjie},
      title        = {{B}alancing dynamic evolution of active sites for urea
                      oxidation in practical scenarios},
      journal      = {Energy $\&$ environmental science},
      volume       = {16},
      number       = {12},
      issn         = {1754-5692},
      address      = {Cambridge},
      publisher    = {RSC Publ.},
      reportid     = {PUBDB-2024-01989},
      pages        = {6015 - 6025},
      year         = {2023},
      abstract     = {Electrochemical urea splitting provides a sustainable and
                      environmentally benign route for facilitating energy
                      conversion. Nonetheless, the sustained efficiency of urea
                      splitting is impeded by a scarcity of active sites during
                      extended operational periods. Herein, an atomic
                      heterostructure engineering strategy is proposed to promote
                      the generation of active species via synthesizing unique
                      Ru–O$_4$ coordinated single atom catalysts anchored on Ni
                      hydroxide (Ru$_1$–Ni(OH)$_2$), with ultralow Ru loading
                      mass of 40.6 μg cm$^{−2}$ on the nickel foam for
                      commercial feasibility. Leveraging in situ spectroscopic
                      characterizations, the structure-performance relationship in
                      low and high urea concentrations was investigated and
                      exhibited extensive universality. The boosted generation of
                      dynamic Ni$^{3+}$ active sites ensures outstanding activity
                      and prominent long-term durability tests in various
                      practical scenarios, including 100 h Zn–urea–air battery
                      operation, 100 h alkaline urine electrolysis, and over 400 h
                      stable hydrogen production in membrane electrode assembly
                      (MEA) system under industrial-level current density.},
      cin          = {DOOR ; HAS-User},
      ddc          = {690},
      cid          = {I:(DE-H253)HAS-User-20120731},
      pnm          = {6G3 - PETRA III (DESY) (POF4-6G3)},
      pid          = {G:(DE-HGF)POF4-6G3},
      experiment   = {EXP:(DE-H253)P-P65-20150101},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:001094835700001},
      doi          = {10.1039/D3EE03258B},
      url          = {https://bib-pubdb1.desy.de/record/607686},
}