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000607686 1001_ $$0P:(DE-HGF)0$$aZhang, Jichao$$b0
000607686 245__ $$aBalancing dynamic evolution of active sites for urea oxidation in practical scenarios
000607686 260__ $$aCambridge$$bRSC Publ.$$c2023
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000607686 520__ $$aElectrochemical urea splitting provides a sustainable and environmentally benign route for facilitating energy conversion. Nonetheless, the sustained efficiency of urea splitting is impeded by a scarcity of active sites during extended operational periods. Herein, an atomic heterostructure engineering strategy is proposed to promote the generation of active species via synthesizing unique Ru–O$_4$ coordinated single atom catalysts anchored on Ni hydroxide (Ru$_1$–Ni(OH)$_2$), with ultralow Ru loading mass of 40.6 μg cm$^{−2}$ on the nickel foam for commercial feasibility. Leveraging in situ spectroscopic characterizations, the structure-performance relationship in low and high urea concentrations was investigated and exhibited extensive universality. The boosted generation of dynamic Ni$^{3+}$ active sites ensures outstanding activity and prominent long-term durability tests in various practical scenarios, including 100 h Zn–urea–air battery operation, 100 h alkaline urine electrolysis, and over 400 h stable hydrogen production in membrane electrode assembly (MEA) system under industrial-level current density. 
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000607686 7001_ $$00000-0003-1629-240X$$aZhu, Jiexin$$b1
000607686 7001_ $$0P:(DE-H253)PIP1085988$$aKang, Liqun$$b2
000607686 7001_ $$0P:(DE-H253)PIP1014745$$aZhang, Qing$$b3
000607686 7001_ $$0P:(DE-HGF)0$$aLiu, Longxiang$$b4
000607686 7001_ $$0P:(DE-HGF)0$$aGuo, Fei$$b5
000607686 7001_ $$0P:(DE-HGF)0$$aLi, Kaiqi$$b6
000607686 7001_ $$0P:(DE-HGF)0$$aFeng, Jianrui$$b7
000607686 7001_ $$0P:(DE-HGF)0$$aXia, Lixue$$b8
000607686 7001_ $$0P:(DE-HGF)0$$aLv, Lei$$b9
000607686 7001_ $$00000-0002-1815-6471$$aZong, Wei$$b10
000607686 7001_ $$00000-0002-1387-9531$$aShearing, Paul R.$$b11
000607686 7001_ $$00000-0002-8545-3126$$aBrett, Dan J. L.$$b12
000607686 7001_ $$00000-0002-4072-6610$$aParkin, Ivan P.$$b13
000607686 7001_ $$0P:(DE-HGF)0$$aSong, Xuedan$$b14$$eCorresponding author
000607686 7001_ $$0P:(DE-HGF)0$$aMai, Liqiang$$b15$$eCorresponding author
000607686 7001_ $$0P:(DE-HGF)0$$aHe, Guanjie$$b16$$eCorresponding author
000607686 773__ $$0PERI:(DE-600)2439879-2$$a10.1039/D3EE03258B$$gVol. 16, no. 12, p. 6015 - 6025$$n12$$p6015 - 6025$$tEnergy & environmental science$$v16$$x1754-5692$$y2023
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