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@ARTICLE{Ye:607627,
      author       = {Ye, Chumei and Lampronti, Giulio I. and McHugh, Lauren N.
                      and Castillo-Blas, Celia and Kono, Ayano and Chen, Celia and
                      Robertson, Georgina P. and Nagle-Cocco, Liam A. V. and Xu,
                      Weidong and Stranks, Samuel D. and Martinez, Valentina and
                      Brekalo, Ivana and Karadeniz, Bahar and Užarević,
                      Krunoslav and Xue, Wenlong and Kolodzeiski, Pascal and Das,
                      Chinmoy and Chater, Philip and Keen, David A. and Dutton,
                      Siân E. and Bennett, Thomas D},
      title        = {{M}echanochemically-induced glass formation from
                      two-dimensional hybrid organic–inorganic perovskites},
      journal      = {Chemical science},
      volume       = {15},
      number       = {19},
      issn         = {2041-6520},
      address      = {Cambridge},
      publisher    = {RSC},
      reportid     = {PUBDB-2024-01963},
      pages        = {7198-7205},
      year         = {2024},
      note         = {Funding sources: Cambridge Research Fellowship
                      $URF\R\211013;$ the Cambridge Trusts and EPSRC Cambridge
                      NanoDTC, EP/S022953/1; EPSRC scholarship, EP/R513180/1; the
                      Leverhulme Trust, Research Project Grant, RPG-2020-005; the
                      Croatian Science Foundation, IP-2020-02-4702; the Royal
                      Society and Tata Group, UF150033; and the EPSRC,
                      EP/V027131/1.},
      abstract     = {Hybrid organic–inorganic perovskites (HOIPs) occupy a
                      prominent position in the field of materials chemistry due
                      to their attractive optoelectronic properties. While
                      extensive work has been done on the crystalline materials
                      over the past decades, the newly reported glasses formed
                      from HOIPs open up a new avenue for perovskite research with
                      their unique structures and functionalities. Melt-quenching
                      is the predominant route to glass formation; however, the
                      absence of a stable liquid state prior to thermal
                      decomposition precludes this method for most HOIPs. In this
                      work, we describe the first mechanochemically-induced
                      crystal-glass transformation of HOIPs as a rapid, green and
                      efficient approach for producing glasses. The amorphous
                      phase was formed from the crystalline phase within 10
                      minutes of ball-milling, and exhibited glass transition
                      behaviour as evidenced by thermal analysis techniques.
                      Time-resolved in situ ball-milling with synchrotron powder
                      diffraction was employed to study the microstructural
                      evolution of amorphisation, which showed that the
                      crystallite size reaches a comminution limit before the
                      amorphisation process is complete, indicating that energy
                      may be further accumulated as crystal defects. Total
                      scattering experiments revealed the limited short-range
                      order of amorphous HOIPs, and their optical properties were
                      studied by ultraviolet-visible (UV-vis) spectroscopy and
                      photoluminescence (PL) spectroscopy.},
      cin          = {DOOR ; HAS-User},
      ddc          = {540},
      cid          = {I:(DE-H253)HAS-User-20120731},
      pnm          = {6G3 - PETRA III (DESY) (POF4-6G3) / FS-Proposal: I-20221330
                      EC (I-20221330-EC)},
      pid          = {G:(DE-HGF)POF4-6G3 / G:(DE-H253)I-20221330-EC},
      experiment   = {EXP:(DE-H253)P-P02.1-20150101},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:38756817},
      UT           = {WOS:001205133800001},
      doi          = {10.1039/D4SC00905C},
      url          = {https://bib-pubdb1.desy.de/record/607627},
}