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@ARTICLE{Herbert:607626,
author = {Herbert, Benedikt and Walpuski, Janis and Stolte, Matthias
and Shoyama, Kazutaka},
title = {{D}esigning {O}rganic π‐{C}onjugated {M}olecules for
{C}rystalline {S}olid {S}olutions:
{A}damantane‐{S}ubstituted {N}aphthalenes},
journal = {ChemPlusChem},
volume = {89},
number = {6},
issn = {2192-6506},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {PUBDB-2024-01962},
pages = {e202300761},
year = {2024},
abstract = {We showcase herein organic crystalline solid solutions
(CSSs) based on the simplest polycyclic aromatic hydrocarbon
(PAH) scaffold, naphthalene, stabilized by dispersion forces
induced by adamantane substitution. High thermal stability
of the host and guest molecules synthesized by
cross-coupling of dibromonaphthalene derivatives and
4-(1-adamantyl)phenyl boronic ester enabled formation of
crystals by sublimation. We could generate binary
monocrystalline solid solution systems proven by X-ray
crystallography, the first system of designed CSSs
stabilized exclusively via dispersion forces with structural
evidence. These observations are additionally supported by
lattice energy calculations and spectroscopic examinations.
For the generation of CSSs, it is of utmost importance that
the host and guest molecules have similar lattice energies
and spatial compatibility. We anticipate that the
thermostable organic CSS design demonstrated herein would be
beneficial for functional materials and further
investigation towards materials with unique properties.},
cin = {DOOR ; HAS-User},
ddc = {540},
cid = {I:(DE-H253)HAS-User-20120731},
pnm = {6G3 - PETRA III (DESY) (POF4-6G3) / FS-Proposal: I-20220939
(I-20220939) / FS-Proposal: I-20230262 (I-20230262)},
pid = {G:(DE-HGF)POF4-6G3 / G:(DE-H253)I-20220939 /
G:(DE-H253)I-20230262},
experiment = {EXP:(DE-H253)P-P11-20150101},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:38259048},
UT = {WOS:001157864300001},
doi = {10.1002/cplu.202300761},
url = {https://bib-pubdb1.desy.de/record/607626},
}