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000607609 1001_ $$0P:(DE-H253)PIP1091370$$aChen, Qing$$b0$$eCorresponding author$$udesy
000607609 245__ $$aHygro-Dynamic and Conductive Actuator That Restructures and Heals by Water
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000607609 520__ $$aThe prospects of endowing stimuli-responsive materials with various life-likebehaviors are promoting the development of intelligent robotic and electronicdevices. However, it is challenging to incorporate stimuli-responsiveactuating and healing capabilities into one single material system. Herein, thedesign and assembly of humidity-responsive thin films composed of poly(3,4-ethylenedioxythiophene):polystyrene sulfonate (PEDOT:PSS) and sodiumcarboxymethyl cellulose (NaCMC) forming a conducting polymer compositethrough a physically cross-linked and hydrogen-bonded supramolecularnetwork are described. Owing to its enhanced dynamics of hydrogen bondingat an elevated humidity, the PEDOT:PSS/NaCMC thin film exhibits a rapidhumidity-responsive actuating performance in an environment with humiditygradient, as well as a repairing function of the structural, mechanical, electrical,and actuating properties after being damaged through a humidifying-dryingcycle. Based on a combined analytical approach, a structural model isproposed for the rearrangement of the thin film when being exposedto stepwise humidity levels at multi-length scales. Due to the structuralrearrangement powered by humidity variations, the film exhibits tunableactuating and healing performance, which makes it a promising candidatematerial for applications in intelligent soft robotics such as artificial muscles.
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000607609 7001_ $$0P:(DE-HGF)0$$aKünniger, Tina$$b1
000607609 7001_ $$0P:(DE-HGF)0$$aSong, Qun$$b2
000607609 7001_ $$0P:(DE-H253)PIP1081802$$aZhang, Kai$$b3
000607609 7001_ $$0P:(DE-H253)PIP1088640$$aChumakov, Andrei$$b4$$udesy
000607609 7001_ $$0P:(DE-H253)PIP1098114$$aBulut, Yusuf$$b5$$udesy
000607609 7001_ $$0P:(DE-H253)PIP1088126$$aHarder, Constantin$$b6$$udesy
000607609 7001_ $$0P:(DE-H253)PIP1007825$$aMüller-Buschbaum, Peter$$b7
000607609 7001_ $$0P:(DE-H253)PIP1003299$$aRoth, Stephan V.$$b8$$eCorresponding author$$udesy
000607609 7001_ $$0P:(DE-H253)PIP1100638$$aBraun, Artur$$b9$$eCorresponding author
000607609 77318 $$2Crossref$$3journal-article$$a10.1002/adfm.202402924$$bWiley$$d2024-05-23$$n38$$tAdvanced Functional Materials$$v34$$x1616-301X$$y2024
000607609 773__ $$0PERI:(DE-600)2039420-2$$a10.1002/adfm.202402924$$gVol. 34, no. 38, p. 2402924$$n38$$p2402924$$tAdvanced functional materials$$v34$$x1616-301X$$y2024
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