Home > Publications database > $J = ^1_2$ pseudospins and $d βˆ’ p$ hybridization in the Kitaev spin liquid candidates $RuX_3$ ( X =Cl, Br, I) > print

001     607542
005     20250715171214.0
024 7 _ |a 10.1103/PhysRevB.109.L180413
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100 1 _ |a Gretarsson, H.
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245 _ _ |a $J = ^1_2$ pseudospins and $d βˆ’ p$ hybridization in the Kitaev spin liquid candidates $RuX_3$ ( X =Cl, Br, I)
260 _ _ |a Woodbury, NY
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520 _ _ |a The recent synthesis of ruthenium trihalides $RuX_3$ (𝑋 = Cl, Br, I) has enlarged the set of material candidates for Kitaev spin liquids. The realization of the Kitaev model necessitates the formation of $J = ^1_2$ pseudospins in the octahedral crystal field. We use Ru $𝐿_3$-edge resonant inelastic x-ray scattering to investigate the evolution of multiplet structures in $RuX_3$. We identified quasielastic magnetic correlations and spin-orbit transitions to the $J = ^3_2$ states without discernible trigonal splitting, thereby validating the $J = ^1_2$ description of magnetism in the $RuX_3$ family. Lineshape broadening in $RuX_3$ provides evidence for its bulk metallicity in the vicinity of a bandwidth-controlled metal-insulator transition. Our results highlight the pivotal role of halogen 𝑝 orbitals in controlling the electronic properties of $RuX_3$.
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700 1 _ |a Fujihara, H.
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700 1 _ |a Sato, F.
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700 1 _ |a Gotou, H.
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700 1 _ |a Imai, Y.
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700 1 _ |a Ohgushi, K.
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700 1 _ |a Keimer, B.
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700 1 _ |a Suzuki, Hakuto
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