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@ARTICLE{Onvlee:607375,
      author       = {Onvlee, Jolijn and Trippel, Sebastian and Küpper, Jochen},
      title        = {{U}ltrafast light-induced dynamics in the microsolvated
                      biomolecular indole chromophore with water},
      reportid     = {PUBDB-2024-01857, arXiv:2103.07171},
      year         = {2022},
      abstract     = {Interactions between proteins and their solvent environment
                      can be studied in a bottom-up approach using hydrogen-bonded
                      chromophore-solvent clusters. The ultrafast dynamics
                      following UV-light-induced electronic excitation of the
                      chromophores, potential radiation damage, and their
                      dependence on solvation are important open questions. The
                      microsolvation effect is challenging to study due to the
                      inherent mix of the produced gas-phase aggregates. We use
                      the electrostatic deflector to spatially separate different
                      molecular species in combination with pump-probe
                      velocity-map-imaging experiments. We demonstrate that this
                      powerful experimental approach reveals intimate details of
                      the UV-induced dynamics in the near-UV-absorbing
                      prototypical biomolecular indole-water system. We determine
                      the time-dependent appearance of the different reaction
                      products and disentangle the occurring ultrafast processes.
                      This approach ensures that the reactants are well-known and
                      that detailed characteristics of the specific reaction
                      products are accessible -- paving the way for the complete
                      chemical-reactivity experiment.},
      cin          = {FS-CFEL-CMI},
      ddc          = {500},
      cid          = {I:(DE-H253)FS-CFEL-CMI-20220405},
      pnm          = {631 - Matter – Dynamics, Mechanisms and Control
                      (POF4-631) / DFG project 390715994 - EXC 2056: CUI: Advanced
                      Imaging of Matter (390715994) / DFG project 194651731 - EXC
                      1074: Hamburger Zentrum für ultraschnelle Beobachtung
                      (CUI): Struktur, Dynamik und Kontrolle von Materie auf
                      atomarer Skala (194651731) / MEDEA - Molecular Electron
                      Dynamics investigated by IntensE Fields and Attosecond
                      Pulses (641789) / COMOTION - Controlling the Motion of
                      Complex Molecules and Particles (614507)},
      pid          = {G:(DE-HGF)POF4-631 / G:(GEPRIS)390715994 /
                      G:(GEPRIS)194651731 / G:(EU-Grant)641789 /
                      G:(EU-Grant)614507},
      experiment   = {EXP:(DE-H253)CFEL-Exp-20150101},
      typ          = {PUB:(DE-HGF)25},
      eprint       = {2103.07171},
      howpublished = {arXiv:2103.07171},
      archivePrefix = {arXiv},
      SLACcitation = {$\%\%CITATION$ = $arXiv:2103.07171;\%\%$},
      pubmed       = {pmid:36460654},
      url          = {https://bib-pubdb1.desy.de/record/607375},
}